{"id":"W1499237562","doi":"10.1063/1.4908130","title":"Partial secular Bloch-Redfield master equation for incoherent excitation of multilevel quantum systems","year":2015,"lang":"en","type":"article","venue":"The Journal of Chemical Physics","topic":"Spectroscopy and Quantum Chemical Studies","field":"Physics and Astronomy","cited_by":50,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Toronto","funders":"U.S. Air Force; Air Force Office of Scientific Research; Canadian Network for Research and Innovation in Machining Technology, Natural Sciences and Engineering Research Council of Canada","keywords":"Master equation; Excited state; Excitation; Density matrix; Dipole; Quantum; Ground state; Basis (linear algebra)","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0007259563,0.0003294867,0.0005327711,0.0005249077,0.0004204419,0.0005537334,0.001268648,0.0007674189,0.002582828],"category_scores_gemma":[0.001312452,0.0002678385,0.0004717249,0.0005222584,0.0008252881,0.001173646,0.0008195778,0.0009009238,0.0003359863],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.001039937,"about_ca_system_score_gemma":0.0009711153,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.002078759,"about_ca_topic_score_gemma":0.002130035,"domain_scores_codex":[0.9997883,0.00005428662,0.000008623872,0.00002324957,0.00009346579,0.0000321243],"domain_scores_gemma":[0.9997126,0.0001354023,0.00003475933,0.00004859217,0.00004798869,0.00002056555],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"theoretical_or_conceptual","study_design_gemma":"simulation_or_modeling","study_design_scores_codex":[0.00003585777,0.00003418501,0.0005681267,0.00006729684,0.00002007895,0.0001235758,0.0002176315,0.3795145,0.01285822,0.594799,0.000766309,0.01099524],"study_design_scores_gemma":[0.000003071444,0.000004896223,0.00006257951,0.000002613018,0.000001281676,0.00001190745,0.000006081003,0.9796438,0.000452867,0.01957532,0.0002313123,0.000004257687],"study_design_candidate":"simulation_or_modeling","study_design_consensus":null,"genre_codex":"methods","genre_gemma":"empirical","genre_scores_codex":[0.08434327,0.0002986226,0.9071606,0.0003318274,0.00002855738,0.00005124665,0.0001533077,0.0001499837,0.00748244],"genre_scores_gemma":[0.7672842,0.0005476648,0.2194381,0.0001781394,0.00004164511,0.0003370873,0.0002404258,0.0001412713,0.01179152],"genre_candidate":"empirical","genre_consensus":null,"teacher_disagreement_score":0.002582828,"threshold_uncertainty_score":0.008640409,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.08468401508365966,"score_gpt":0.2991748572160848,"score_spread":0.2144908421324251,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}