{"id":"W2009066441","doi":"10.1016/j.jcat.2013.10.008","title":"Mechanical modulation of reaction rates in electrocatalysis","year":2013,"lang":"en","type":"article","venue":"Journal of Catalysis","topic":"Electrocatalysts for Energy Conversion","field":"Energy","cited_by":60,"is_retracted":false,"has_abstract":false,"ca_institutions":"University of Guelph","funders":"","keywords":"Chemistry; Overpotential; Electrocatalyst; Enthalpy; Exchange current density; Catalysis; Tafel equation; Ab initio; Reactivity (psychology); Thermodynamics; Hydrogen; Reaction rate; Reaction rate constant; Electrochemistry; Physical chemistry; Electrode; Kinetics","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0006242719,0.0001562769,0.0005199008,0.000892709,0.00003181268,0.00001946006,0.0002261346,0.0001379406,0.0001527891],"category_scores_gemma":[0.0002811096,0.0001357011,0.0003343033,0.001167958,0.00002952909,0.0008804594,0.00003298135,0.0002575667,0.00004265227],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0003275646,"about_ca_system_score_gemma":0.00008743356,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.002435565,"about_ca_topic_score_gemma":0.0006063959,"domain_scores_codex":[0.9978935,0.0001005275,0.0009707374,0.0001699447,0.000623756,0.000241585],"domain_scores_gemma":[0.9979957,0.0001102735,0.0008631399,0.0002956519,0.0006440864,0.00009118487],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00008952815,0.0001412973,0.0008177686,0.00001404927,0.0002576301,0.000007903878,0.00009794383,0.002768573,0.9796593,0.0009889101,0.0001403477,0.01501675],"study_design_scores_gemma":[0.0008935718,0.0002597373,0.01178481,0.00004652024,0.000290533,0.00008455817,0.0001663549,0.006913157,0.9737285,0.005133186,0.0005016461,0.0001974278],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9978054,0.0001662709,0.0008006287,0.000309446,0.00008701489,0.00005569543,1.73995e-7,0.00001194773,0.0007634088],"genre_scores_gemma":[0.9990641,0.0001080453,0.0004978669,0.00002607507,0.00009324637,0.00000525892,0.00003266176,0.00002138398,0.0001513085],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.01481932,"threshold_uncertainty_score":0.5533732,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.006916378825434461,"score_gpt":0.2260437147736918,"score_spread":0.2191273359482573,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}