{"id":"W2093409513","doi":"10.1039/c3cp52630e","title":"Density dependence of the yield of hydrated electrons in the low-LET radiolysis of supercritical water at 400 °C: influence of the geminate recombination of subexcitation-energy electrons prior to thermalization","year":2013,"lang":"en","type":"article","venue":"Physical Chemistry Chemical Physics","topic":"Subcritical and Supercritical Water Processes","field":"Engineering","cited_by":11,"is_retracted":false,"has_abstract":true,"ca_institutions":"Université de Sherbrooke","funders":"Natural Resources Canada; Natural Sciences and Engineering Research Council of Canada","keywords":"Radiolysis; Thermalisation; Solvated electron; Supercritical fluid; Electron; Chemistry; Yield (engineering); Range (aeronautics); Picosecond; Electron density; Atomic physics; Materials science; Physical chemistry; Aqueous solution; Physics; Laser; Nuclear physics","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0003475022,0.0003453587,0.0002862582,0.0002249367,0.0002435557,0.0003238003,0.0004407052,0.0002851942,0.0009992641],"category_scores_gemma":[0.001439201,0.0002712061,0.0002310804,0.0002332811,0.0004910892,0.0006092655,0.0002383273,0.0004803812,0.0001518269],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.001042618,"about_ca_system_score_gemma":0.0004919014,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.005813213,"about_ca_topic_score_gemma":0.003804774,"domain_scores_codex":[0.9998947,0.00001155779,0.000004740186,0.00002147147,0.00004226752,0.0000251618],"domain_scores_gemma":[0.9995964,0.0002572338,0.00003632156,0.00001664806,0.00007563402,0.00001769667],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0006282055,0.000137161,0.01378828,0.0003581555,0.00007583613,0.0004163023,0.0005689918,0.4521827,0.5149626,0.005503467,0.000247358,0.01113103],"study_design_scores_gemma":[0.00003413497,0.0001857259,0.004427623,0.00001409231,0.0000301535,0.00004675738,0.0001011277,0.4718857,0.5221857,0.0005898383,0.0004700536,0.00002903819],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.992859,0.0001296071,0.005759492,0.00004047326,0.00000422195,0.00001914328,0.00009219929,0.00006567781,0.001030104],"genre_scores_gemma":[0.9983771,0.0001328144,0.001072446,0.000008511385,7.619496e-7,0.00001561898,0.00007085779,0.00001671818,0.000305291],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.005813213,"threshold_uncertainty_score":0.01155877,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.003914189325193818,"score_gpt":0.1823527870126224,"score_spread":0.1784385976874285,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}