{"id":"W2096828089","doi":"10.1139/cjc-2014-0048","title":"Size-independent organosilane functionalization of silicon nanocrystals using Wilkinson’s catalyst","year":2014,"lang":"en","type":"article","venue":"Canadian Journal of Chemistry","topic":"Silicon Nanostructures and Photoluminescence","field":"Materials Science","cited_by":16,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Alberta","funders":"Natural Sciences and Engineering Research Council of Canada; University of Alberta","keywords":"Surface modification; Silanes; Chemistry; Steric effects; Catalysis; Quenching (fluorescence); Silicon; Nanocrystal; Photoluminescence; X-ray photoelectron spectroscopy; Photochemistry; Hydrosilylation; Rhodium; Chemical engineering; Nanotechnology; Physical chemistry; Organic chemistry; Silane; Fluorescence; Materials science","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":true,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":["insufficient_payload"],"consensus_categories":[],"category_scores_codex":[0.0002815963,0.0001198544,0.0002504194,0.00004956091,0.00008766431,0.00004812311,0.0002861641,0.0001090414,0.00194497],"category_scores_gemma":[0.0004077843,0.0001119321,0.00007505273,0.0001395307,0.0001100541,0.0001241477,0.00001202054,0.000102093,0.000002877793],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0001400562,"about_ca_system_score_gemma":0.0009529091,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.002112755,"about_ca_topic_score_gemma":0.0007288939,"domain_scores_codex":[0.9989059,0.00003083913,0.0004470291,0.0001381222,0.0002611738,0.0002169434],"domain_scores_gemma":[0.99855,0.00006439596,0.0004869106,0.0001955056,0.0003353451,0.0003678575],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00001452257,0.00000563357,0.0072695,0.00006734485,0.000007740478,0.00001308754,0.00009898858,0.0002463347,0.9917697,0.00001049896,0.0004491545,0.00004750535],"study_design_scores_gemma":[0.0003072132,0.00002423242,0.003029402,0.00009193814,0.00002435697,0.000465946,0.00007787625,0.0000627136,0.9939827,0.0001091268,0.0017097,0.0001147902],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9987832,0.0002172294,0.0001041389,0.0000553765,0.0004767154,0.00003841884,0.00003933064,0.000003843706,0.000281748],"genre_scores_gemma":[0.9993701,0.000003347808,0.000100546,0.00007936409,0.0002702656,3.983531e-7,0.000005967194,0.00001300773,0.000156994],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.004240098,"threshold_uncertainty_score":0.9989674,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.007876170016707748,"score_gpt":0.2048434282390242,"score_spread":0.1969672582223164,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}