{"id":"W2098527861","doi":"10.1126/science.1217745","title":"The Role of Driving Energy and Delocalized States for Charge Separation in Organic Semiconductors","year":2012,"lang":"en","type":"article","venue":"Science","topic":"Organic Electronics and Photovoltaics","field":"Engineering","cited_by":1176,"is_retracted":false,"has_abstract":true,"ca_institutions":"","funders":"Engineering and Physical Sciences Research Council; Fonds De La Recherche Scientifique - FNRS; Corpus Christi College, University of Cambridge; Natural Sciences and Engineering Research Council of Canada; Alexander von Humboldt-Stiftung; Nederlandse Organisatie voor Wetenschappelijk Onderzoek; Stichting voor Fundamenteel Onderzoek der Materie","keywords":"Delocalized electron; Exciton; Photoinduced charge separation; Picosecond; Excited state; Chemical physics; Intermolecular force; Atomic physics; Electron; Organic semiconductor; Molecular physics; Charge carrier; Dissociation (chemistry); Chemistry; Materials science; Optoelectronics; Condensed matter physics; Physics; Photocatalysis; Molecule; Quantum mechanics","routes":{"ca_aff":false,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":true},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001163198,0.0001503327,0.00008637238,0.0001721249,0.0004272543,0.0004753914,0.0002651626,0.0002399524,0.0009144081],"category_scores_gemma":[0.0002683938,0.0001400171,0.00008295565,0.00008554825,0.000526159,0.0005990432,0.0002726941,0.0004454963,0.0001117058],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0004372081,"about_ca_system_score_gemma":0.0001807554,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.000242414,"about_ca_topic_score_gemma":0.0003950702,"domain_scores_codex":[0.9999694,0.000004735967,0.000001437251,0.000007359095,0.000008034253,0.000009151932],"domain_scores_gemma":[0.9999038,0.00005450678,0.00001237632,0.000008155695,0.00000710511,0.00001394805],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0001796975,0.0001192724,0.001693478,0.0002006692,0.00001408916,0.0002420341,0.0002744842,0.009812763,0.924015,0.04217608,0.000141638,0.02113071],"study_design_scores_gemma":[0.00004049058,0.0004636578,0.003755755,0.00002553139,0.00002483957,0.0003428512,0.0003321269,0.07116554,0.9009543,0.02082266,0.002029008,0.00004326578],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9883052,0.001051358,0.008758011,0.0001158566,0.00001448203,0.000008570454,0.00001417337,0.00004743613,0.00168492],"genre_scores_gemma":[0.9988292,0.0001845782,0.000712801,0.00000912997,0.000002055369,0.000003977736,0.000005306271,0.000004438484,0.0002485034],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0009144081,"threshold_uncertainty_score":0.003172219,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.004187192002907641,"score_gpt":0.2186658554602308,"score_spread":0.2144786634573232,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}