{"id":"W2126705766","doi":"10.1038/nature12044","title":"Mapping molecular motions leading to charge delocalization with ultrabright electrons","year":2013,"lang":"en","type":"article","venue":"Nature","topic":"Advanced Electron Microscopy Techniques and Applications","field":"Biochemistry, Genetics and Molecular Biology","cited_by":283,"is_retracted":false,"has_abstract":false,"ca_institutions":"University of Toronto","funders":"Natural Sciences and Engineering Research Council of Canada","keywords":"Femtosecond; Ultrafast electron diffraction; Picosecond; Dephasing; Ultrashort pulse; Delocalized electron; Electron; Femtochemistry; Excitation; Chemical physics; Materials science; Diffraction; Laser; Temporal resolution; Electron diffraction; Molecular physics; Optics; Chemistry; Physics; Condensed matter physics","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.00002939327,0.0001241948,0.0000798429,0.00005051708,0.0001162245,0.00002660955,0.0001384084,0.0003787601,0.00003772102],"category_scores_gemma":[0.00001293093,0.0001090221,0.00003260014,0.0002630306,0.00002061894,0.000006647277,0.00002385945,0.000399822,0.00003911977],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.00002538804,"about_ca_system_score_gemma":0.00002905304,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.000004667043,"about_ca_topic_score_gemma":0.000009397492,"domain_scores_codex":[0.9992636,0.00001143109,0.00009308688,0.0002902169,0.00007660963,0.0002650041],"domain_scores_gemma":[0.9995195,0.000001969775,0.00003552814,0.0002485584,0.0001189298,0.00007557461],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.000002806757,0.00001913463,0.0000832063,0.000003500915,0.0000119699,3.077484e-7,0.0000122303,0.0001383041,0.9881767,0.00231369,0.008607147,0.0006310269],"study_design_scores_gemma":[0.00008535424,0.0001045062,0.0001731765,0.00001194588,0.000004700828,0.00001198516,0.00001053905,0.00006493221,0.8881225,0.0002753303,0.1109754,0.0001595854],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"methods","genre_gemma":"empirical","genre_scores_codex":[0.2560178,0.0004192822,0.7403499,0.001285754,0.00001447613,0.0004954647,0.00001025538,0.00006087752,0.001346252],"genre_scores_gemma":[0.9771111,0.0000439568,0.01867409,0.00222713,0.0000662382,0.0002204313,0.0002447924,0.00003056179,0.001381715],"genre_candidate":"empirical","genre_consensus":null,"teacher_disagreement_score":0.7216758,"threshold_uncertainty_score":0.4445791,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.002672801119410807,"score_gpt":0.268334239425789,"score_spread":0.2656614383063782,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}