{"id":"W2281093366","doi":"10.1039/c5cy01524c","title":"Active phase distribution changes within a catalyst particle during Fischer–Tropsch synthesis as revealed by multi-scale microscopy","year":2016,"lang":"en","type":"article","venue":"Catalysis Science & Technology","topic":"Catalysts for Methane Reforming","field":"Chemical Engineering","cited_by":54,"is_retracted":false,"has_abstract":true,"ca_institutions":"Canadian Light Source (Canada); Saskatoon Medical Imaging","funders":"National Research Council Canada; Nederlandse Organisatie voor Wetenschappelijk Onderzoek; Western Economic Diversification Canada; Canadian Institutes of Health Research; Office of Science; U.S. Department of Energy; European Commission; Universiteit Utrecht; Canadian Light Source; Natural Sciences and Engineering Research Council of Canada; University of Saskatchewan; SLAC National Accelerator Laboratory; Shell","keywords":"Fischer–Tropsch process; Catalysis; Chemical engineering; Particle (ecology); Phase (matter); Materials science; Particle-size distribution; Chemistry; Nanotechnology; Particle size; Organic chemistry; Geology; Engineering; Selectivity","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001474769,0.0002236001,0.000117393,0.0003407203,0.0001415876,0.0002492675,0.0002135662,0.0002578016,0.0007232485],"category_scores_gemma":[0.0001683902,0.0002353114,0.0001070617,0.0001127465,0.0003367322,0.0003381058,0.0001906544,0.0003484853,0.0001628612],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002336127,"about_ca_system_score_gemma":0.0001041497,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0008722666,"about_ca_topic_score_gemma":0.001267065,"domain_scores_codex":[0.9999272,0.000004648383,0.000004508101,0.00002304343,0.00002280553,0.00001780662],"domain_scores_gemma":[0.9998662,0.00004914897,0.00003478337,0.00001773003,0.00001825807,0.00001385248],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00002200367,0.000002693267,0.0001492328,0.000009154719,0.000001662135,0.00002614169,0.0000215459,0.00005022545,0.9987059,0.00005939881,0.00001150463,0.0009405712],"study_design_scores_gemma":[0.000003437707,0.00002784106,0.00421446,0.000001523147,0.000005860533,0.0001144737,0.00002264732,0.001644655,0.9935188,0.00002470805,0.0004165352,0.000005105893],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9823236,0.0007910142,0.01511745,0.00006623497,0.00001848204,0.00001926647,0.0001398103,0.0001310565,0.001393007],"genre_scores_gemma":[0.9904153,0.0003738019,0.00768595,0.00001287415,0.000009666619,0.00002007273,0.00008565453,0.00002951547,0.001367081],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0008722666,"threshold_uncertainty_score":0.002419472,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.00924776180872025,"score_gpt":0.2747099507921932,"score_spread":0.265462188983473,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}