{"id":"W2322812680","doi":"10.1021/jp5090444","title":"Short-Time Dynamics at a Conical Intersection in High-Harmonic Spectroscopy","year":2014,"lang":"en","type":"article","venue":"The Journal of Physical Chemistry A","topic":"Laser-Matter Interactions and Applications","field":"Physics and Astronomy","cited_by":13,"is_retracted":false,"has_abstract":true,"ca_institutions":"Steacie Institute for Molecular Sciences; University of Ottawa","funders":"","keywords":"Conical intersection; Autocorrelation; High harmonic generation; Harmonics; Physics; Harmonic; Vibronic coupling; Atomic physics; Spectroscopy; Wave packet; Laser; Population; Excited state; Optics; Quantum mechanics","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0007162587,0.0001652229,0.0002120472,0.0004414589,0.0004432912,0.0005127686,0.0008457248,0.0005332235,0.000789551],"category_scores_gemma":[0.001740162,0.0002236862,0.0002048271,0.0005515027,0.0008939046,0.0009517373,0.0003669383,0.0006764956,0.00009947813],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0008752513,"about_ca_system_score_gemma":0.0007427237,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.002678864,"about_ca_topic_score_gemma":0.002717581,"domain_scores_codex":[0.9998325,0.00003206093,0.000005272664,0.0000187725,0.00007546382,0.00003589805],"domain_scores_gemma":[0.9994337,0.000326983,0.00006184084,0.00007117429,0.0000616914,0.00004452521],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"simulation_or_modeling","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0003423358,0.0003018134,0.007216617,0.00014113,0.00003229521,0.0004539507,0.0006880461,0.6218473,0.1618938,0.1794634,0.0003409329,0.02727828],"study_design_scores_gemma":[0.000008755841,0.00004099702,0.001149239,0.000004330051,0.000002815415,0.00004168717,0.00004614446,0.9655675,0.02595828,0.006906109,0.0002524912,0.0000216704],"study_design_candidate":"bench_or_experimental","study_design_consensus":null,"genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.8086621,0.0001436414,0.1886366,0.00007379498,0.000009970735,0.00002345847,0.0000371126,0.0001845982,0.002228784],"genre_scores_gemma":[0.9863409,0.0000528079,0.01329563,0.000004733758,0.000002043003,0.00001031541,0.00001940679,0.00001464832,0.0002596083],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.002678864,"threshold_uncertainty_score":0.006350398,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.004684096072661865,"score_gpt":0.2481059236529985,"score_spread":0.2434218275803366,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}