{"id":"W2333112136","doi":"10.1021/ac302789c","title":"Unraveling the Mechanism of Electrospray Ionization","year":2012,"lang":"en","type":"article","venue":"Analytical Chemistry","topic":"Mass Spectrometry Techniques and Applications","field":"Chemistry","cited_by":712,"is_retracted":false,"has_abstract":true,"ca_institutions":"Western University","funders":"Natural Sciences and Engineering Research Council of Canada; Canada Research Chairs","keywords":"Chemistry; Electrospray ionization; Electrospray; Extractive electrospray ionization; Ionization; Ion; Mass spectrometry; Residue (chemistry); Analyte; Evaporation; Analytical Chemistry (journal); Chromatography; Polymer; Sample preparation in mass spectrometry; Organic chemistry; Thermodynamics","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.001663452,0.001174279,0.0005550869,0.0007940839,0.0004997741,0.001610768,0.00166983,0.001474051,0.002832021],"category_scores_gemma":[0.001742902,0.0005312212,0.0004586551,0.0005914228,0.001719358,0.005201202,0.00106639,0.002793499,0.001706652],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0009328546,"about_ca_system_score_gemma":0.00110488,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00055554,"about_ca_topic_score_gemma":0.0003700709,"domain_scores_codex":[0.9994255,0.00007660945,0.00004210666,0.0001374023,0.0002482004,0.00007022265],"domain_scores_gemma":[0.9993056,0.000204719,0.0001098359,0.00007640342,0.0002481415,0.00005523501],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0003153661,0.0001854193,0.001693525,0.002448886,0.00007401726,0.001742744,0.0003464093,0.00286426,0.6868654,0.1318191,0.006824342,0.1648205],"study_design_scores_gemma":[0.00008443266,0.0007668054,0.002172063,0.000511247,0.00007759356,0.004546819,0.0002484074,0.03981955,0.6803969,0.06402706,0.207125,0.0002241429],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"methods","genre_gemma":"empirical","genre_scores_codex":[0.1555224,0.2533599,0.5232641,0.01849665,0.00427729,0.0005087822,0.0006992697,0.001848736,0.04202284],"genre_scores_gemma":[0.6609531,0.1666119,0.1430588,0.003120356,0.00240696,0.000327632,0.0008826437,0.000223788,0.02241481],"genre_candidate":"empirical","genre_consensus":null,"teacher_disagreement_score":0.002832021,"threshold_uncertainty_score":0.009474039,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.0120968106592,"score_gpt":0.2593998392949904,"score_spread":0.2473030286357904,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}