{"id":"W2469687854","doi":"10.1364/up.2002.wd15","title":"Nonlinear Optical Probes of Vibrational Motion at Interfaces.","year":2002,"lang":"en","type":"article","venue":"","topic":"Spectroscopy and Quantum Chemical Studies","field":"Physics and Astronomy","cited_by":0,"is_retracted":false,"has_abstract":true,"ca_institutions":"Simon Fraser University","funders":"","keywords":"Femtosecond; Excitation; Intermolecular force; Raman spectroscopy; Molecular vibration; Raman scattering; Materials science; Sum-frequency generation; Molecular physics; Frequency domain; Molecule; Nonlinear optics; Atomic physics; Laser; Optics; Physics","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001931692,0.0003440544,0.0001246593,0.0002526799,0.0002474701,0.0002898407,0.0003327416,0.0005002951,0.003043673],"category_scores_gemma":[0.000229009,0.0001548658,0.00009732335,0.0001528317,0.0004280356,0.000594574,0.0003081291,0.0008833252,0.0008559308],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002963589,"about_ca_system_score_gemma":0.0001486202,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0003763509,"about_ca_topic_score_gemma":0.000794694,"domain_scores_codex":[0.9998676,0.00001534523,0.000002627969,0.00002665579,0.00006714073,0.00002064256],"domain_scores_gemma":[0.9998643,0.00004745409,0.00002878648,0.00001176968,0.00002276455,0.00002481372],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00003875441,0.00002171954,0.0002288555,0.0001593108,0.000006214208,0.00002718306,0.00002898229,0.00009088862,0.9804078,0.001694935,0.0004918967,0.01680351],"study_design_scores_gemma":[0.00002100551,0.0002056342,0.002653773,0.00002164931,0.00002288289,0.0005656432,0.00005917923,0.003414513,0.9581392,0.001994571,0.03288171,0.00002016129],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.6453099,0.07105669,0.2264796,0.001797496,0.000879568,0.0002083767,0.001056326,0.001799731,0.05141241],"genre_scores_gemma":[0.8792611,0.01176227,0.08491606,0.000621281,0.0001478828,0.0002148194,0.0005550591,0.00005959888,0.02246185],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.003043673,"threshold_uncertainty_score":0.01018214,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01635635650962911,"score_gpt":0.2412935392948208,"score_spread":0.2249371827851917,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}