{"id":"W2569358455","doi":"10.1149/2.1111702jes","title":"Transition Metal Dissolution, Ion Migration, Electrocatalytic Reduction and Capacity Loss in Lithium-Ion Full Cells","year":2017,"lang":"en","type":"article","venue":"Journal of The Electrochemical Society","topic":"Advancements in Battery Materials","field":"Engineering","cited_by":485,"is_retracted":false,"has_abstract":true,"ca_institutions":"","funders":"Argonne National Laboratory; Basic Energy Sciences; Dalhousie University; Office of Science; University of Chicago; U.S. Department of Energy","keywords":"Dissolution; Capacity loss; Electrolyte; Lithium (medication); Ion; Oxide; Transition metal; Fade; Electrode; Chemistry; Interphase; Materials science; Inorganic chemistry; Chemical engineering; Catalysis; Physical chemistry","routes":{"ca_aff":false,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":true},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001541758,0.0002268718,0.0002669684,0.0002480432,0.0001554056,0.00039219,0.0006191933,0.0003768278,0.0007253088],"category_scores_gemma":[0.0004134493,0.0001761773,0.0001590132,0.0002948579,0.0004167022,0.0005668346,0.0002408389,0.0003749128,0.0001748448],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0005863659,"about_ca_system_score_gemma":0.0002124052,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.002051053,"about_ca_topic_score_gemma":0.001831063,"domain_scores_codex":[0.9998763,0.000007110547,0.000009854071,0.0000212268,0.00006615171,0.00001932005],"domain_scores_gemma":[0.9998822,0.0000332555,0.00002856005,0.0000129908,0.00003259046,0.00001036487],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0002839182,0.00003939125,0.004748418,0.0001183317,0.00001119799,0.0002649381,0.00009250639,0.001672169,0.9792069,0.000462975,0.0001318325,0.01296748],"study_design_scores_gemma":[0.000004647168,0.0001316897,0.006507518,0.000005938374,0.000008172618,0.0002747934,0.00006792785,0.008552992,0.983643,0.000205265,0.0005907198,0.000007228747],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9933708,0.001535009,0.003757086,0.00009286938,0.00000806682,0.00001554567,0.0002045666,0.0001429824,0.0008731334],"genre_scores_gemma":[0.9981869,0.0003659302,0.0007563116,0.0000137046,0.000001807924,0.00001028839,0.00008662972,0.000007242365,0.0005711812],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.002051053,"threshold_uncertainty_score":0.004254341,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.008386794110124792,"score_gpt":0.2223833966486547,"score_spread":0.2139966025385299,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}