{"id":"W2622335491","doi":"10.1021/acs.chemrev.6b00770","title":"Capturing Chemistry in Action with Electrons: Realization of Atomically Resolved Reaction Dynamics","year":2017,"lang":"en","type":"review","venue":"Chemical Reviews","topic":"Advanced Electron Microscopy Techniques and Applications","field":"Biochemistry, Genetics and Molecular Biology","cited_by":171,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Toronto","funders":"Division of Chemical, Bioengineering, Environmental, and Transport Systems; Defense Threat Reduction Agency; Max-Planck-Gesellschaft; Russian Foundation for Basic Research","keywords":"Chemistry; Attosecond; Reaction dynamics; Femtosecond; Temporal resolution; Electron; Chemical physics; Nanotechnology; Atomic physics; Molecule; Physics; Optics; Quantum mechanics; Laser","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0004169829,0.0002399519,0.000322462,0.0002352006,0.0003504909,0.0009719099,0.0006364817,0.0007370849,0.0022826],"category_scores_gemma":[0.0006660869,0.0002470022,0.0002575925,0.0002011062,0.001332457,0.002407702,0.001055659,0.001477774,0.0004463179],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0004338577,"about_ca_system_score_gemma":0.0002530041,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0003218965,"about_ca_topic_score_gemma":0.0002965927,"domain_scores_codex":[0.9998577,0.00002806598,0.000006901076,0.00003095046,0.00005166131,0.00002482889],"domain_scores_gemma":[0.9998197,0.00009721406,0.00001675334,0.00003268547,0.00001720805,0.00001647243],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"theoretical_or_conceptual","study_design_gemma":"not_applicable","study_design_scores_codex":[0.0002084185,0.00009264509,0.0009748476,0.0009331043,0.0000479388,0.0005629429,0.0009041447,0.01283435,0.2885005,0.5973386,0.004334989,0.09326752],"study_design_scores_gemma":[0.0001723398,0.0004991234,0.001782366,0.0003268756,0.00007659946,0.0008692104,0.0006656362,0.1389635,0.3158086,0.3682096,0.1724802,0.0001459371],"study_design_candidate":"not_applicable","study_design_consensus":null,"genre_codex":"methods","genre_gemma":"review","genre_scores_codex":[0.3708948,0.04862188,0.4753505,0.007809851,0.00215906,0.00018196,0.0004885521,0.001327262,0.09316622],"genre_scores_gemma":[0.90793,0.0131774,0.07292834,0.0006414031,0.0001765841,0.00009727835,0.000128842,0.00005848331,0.004861675],"genre_candidate":"review","genre_consensus":null,"teacher_disagreement_score":0.0022826,"threshold_uncertainty_score":0.007636011,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.05352750226907015,"score_gpt":0.4199547067551842,"score_spread":0.366427204486114,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}