{"id":"W2793566282","doi":"10.1002/advs.201700732","title":"Tailoring Surface Frustrated Lewis Pairs of In<sub>2</sub>O<sub>3−</sub><i><sub>x</sub></i>(OH)<sub>y</sub> for Gas‐Phase Heterogeneous Photocatalytic Reduction of CO<sub>2</sub> by Isomorphous Substitution of In<sup>3+</sup> with Bi<sup>3+</sup>","year":2018,"lang":"en","type":"article","venue":"Advanced Science","topic":"Advanced Photocatalysis Techniques","field":"Energy","cited_by":132,"is_retracted":false,"has_abstract":true,"ca_institutions":"Dalhousie University; University of Toronto","funders":"Basic Energy Sciences; Natural Sciences and Engineering Research Council of Canada; Ontario Ministry of Research, Innovation and Science; U.S. Department of Energy; Ministero dello Sviluppo Economico; Canadian Light Source","keywords":"Lewis acids and bases; Frustrated Lewis pair; Chemistry; Steric effects; Heterolysis; Photocatalysis; Catalysis; Density functional theory; Borane; Reactivity (psychology); Oxide; Hydride; Crystallography; Stereochemistry; Computational chemistry; Organic chemistry","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":["metaepi_narrow","sts"],"consensus_categories":["metaepi_narrow"],"category_scores_codex":[0.003004479,0.002334899,0.003155,0.002387986,0.0009980946,0.0002113756,0.002689305,0.001026556,0.00001276581],"category_scores_gemma":[0.001201773,0.002541008,0.0007680022,0.009510769,0.006559525,0.004486993,0.000608319,0.001509086,0.00007501044],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.002011945,"about_ca_system_score_gemma":0.001499676,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0005146457,"about_ca_topic_score_gemma":0.00133798,"domain_scores_codex":[0.9841098,0.000565895,0.00433402,0.004345399,0.00304067,0.00360423],"domain_scores_gemma":[0.9889082,0.0007665923,0.003248456,0.003580093,0.002450274,0.001046408],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.002338382,0.001451603,0.0004349708,0.0004604378,0.0001640147,0.0000822251,0.001256475,0.1988804,0.7798119,0.0001268084,0.0001032498,0.01488956],"study_design_scores_gemma":[0.006232632,0.003118254,0.0001551824,0.001377415,0.0003247163,0.0002970696,0.001073082,0.0249164,0.958728,0.001260276,0.0001479315,0.002369051],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9788484,0.0006240482,0.01301094,0.00005325255,0.0004035009,0.005425325,0.0006909146,0.0008110774,0.0001325305],"genre_scores_gemma":[0.9923391,0.001622226,0.003355749,0.0001115244,0.0001977251,0.001232903,0.0006730484,0.000460164,0.000007608096],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.1789161,"threshold_uncertainty_score":0.9989389,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01493938510286613,"score_gpt":0.2671676287160583,"score_spread":0.2522282436131921,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}