{"id":"W2805373389","doi":"10.1039/c8sc00293b","title":"Striking the right balance of intermolecular coupling for high-efficiency singlet fission","year":2018,"lang":"en","type":"article","venue":"Chemical Science","topic":"Molecular Spectroscopy and Structure","field":"Chemistry","cited_by":127,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Toronto; Toronto Public Health","funders":"Division of Chemistry; Division of Materials Research; National Institute of General Medical Sciences; Natural Sciences and Engineering Research Council of Canada; Basic Energy Sciences; Materials Research Science and Engineering Center, Harvard University; Princeton Center for Complex Materials; U.S. Department of Energy; National Institutes of Health; National Science Foundation","keywords":"Singlet fission; Intermolecular force; Balance (ability); Coupling (piping); Fission; Singlet state; Detailed balance; Chemistry; Chemical physics; Physics; Materials science; Atomic physics; Nuclear physics; Quantum mechanics; Medicine; Molecule; Organic chemistry; Physical medicine and rehabilitation; Neutron","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0003101403,0.0004075846,0.0002992589,0.0001690756,0.0003642274,0.0005905133,0.0002497261,0.0003204198,0.001569554],"category_scores_gemma":[0.0006602732,0.0001904796,0.0001551777,0.0001680033,0.0004574519,0.0008522353,0.0004699467,0.0007780623,0.0005211525],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002963456,"about_ca_system_score_gemma":0.0002930092,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0002539716,"about_ca_topic_score_gemma":0.0008440615,"domain_scores_codex":[0.9997661,0.00002882859,0.00002022401,0.00006421982,0.000078864,0.00004170642],"domain_scores_gemma":[0.9995983,0.0001599879,0.00008477688,0.00004818506,0.00005717356,0.00005161975],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00003701512,0.00003205307,0.0003206966,0.0000922286,0.000007354609,0.00008175436,0.00006732142,0.0009409299,0.9924124,0.002343771,0.00005963483,0.003604878],"study_design_scores_gemma":[0.00001680532,0.0002468617,0.001053885,0.00001738278,0.00001132277,0.0001336356,0.00008557347,0.007236048,0.9875163,0.001103096,0.002567776,0.00001126233],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9611101,0.001167568,0.02862276,0.0003135057,0.0000592778,0.00003868479,0.00006260613,0.0001694247,0.008456184],"genre_scores_gemma":[0.9929851,0.0004265178,0.00577129,0.0000516576,0.0000121982,0.00002134358,0.00003717509,0.00004198472,0.0006526513],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.001569554,"threshold_uncertainty_score":0.005250633,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.005450893247918216,"score_gpt":0.2553918052363088,"score_spread":0.2499409119883906,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}