{"id":"W2935876896","doi":"10.1002/anie.201903613","title":"Efficient Electrochemical Reduction of CO<sub>2</sub> to HCOOH over Sub‐2 nm SnO<sub>2</sub> Quantum Wires with Exposed Grain Boundaries","year":2019,"lang":"en","type":"article","venue":"Angewandte Chemie International Edition","topic":"CO2 Reduction Techniques and Catalysts","field":"Energy","cited_by":417,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Alberta","funders":"National Research Foundation","keywords":"Electrochemistry; Materials science; Grain boundary; Reactivity (psychology); Faraday efficiency; Quantum dot; Density functional theory; Nanoparticle; Nanotechnology; Electrode; Chemistry; Physical chemistry; Metallurgy; Computational chemistry","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":["metaepi_narrow"],"consensus_categories":[],"category_scores_codex":[0.0002403669,0.0003505041,0.0003583067,0.0003256739,0.0001394326,0.0001383754,0.0002864194,0.0002302538,0.0001676675],"category_scores_gemma":[0.00009740773,0.000344523,0.0002023623,0.0004091149,0.0002383769,0.0002735567,0.00007693722,0.0003017251,0.00007725809],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0005079561,"about_ca_system_score_gemma":0.0001791541,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0001257786,"about_ca_topic_score_gemma":0.00006564147,"domain_scores_codex":[0.9974393,0.00003618516,0.0005552386,0.0006323258,0.0009461145,0.0003908337],"domain_scores_gemma":[0.9985261,0.00004989408,0.000348939,0.0003798241,0.000543438,0.0001517991],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0008948387,0.000239761,0.00004897197,0.00004788107,0.0001277383,0.000004091987,0.0002975646,0.0001471532,0.9746464,0.003284997,0.01868355,0.00157702],"study_design_scores_gemma":[0.0008818305,0.0003011978,0.0004263448,0.0001803758,0.00004748569,0.00008484798,0.0001772644,0.0002117137,0.9887001,0.00119236,0.00739643,0.0004000811],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9922391,0.00006177973,0.003391728,0.0007141486,0.00163838,0.0003908051,0.00008924206,0.0002376497,0.001237147],"genre_scores_gemma":[0.9966005,0.00006578327,0.0001238983,0.0001495174,0.00126453,0.0001568831,0.00146379,0.00006195475,0.0001131428],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.01405364,"threshold_uncertainty_score":0.9999007,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.007212034682579533,"score_gpt":0.2331104518694249,"score_spread":0.2258984171868454,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}