{"id":"W3039100120","doi":"10.1021/acs.analchem.0c02290","title":"Formation of Gaseous Proteins via the Ion Evaporation Model (IEM) in Electrospray Mass Spectrometry","year":2020,"lang":"en","type":"article","venue":"Analytical Chemistry","topic":"Mass Spectrometry Techniques and Applications","field":"Chemistry","cited_by":48,"is_retracted":false,"has_abstract":true,"ca_institutions":"Western University","funders":"Natural Sciences and Engineering Research Council of Canada","keywords":"Chemistry; Electrospray; Ion; Mass spectrometry; Electrospray ionization; Ion-mobility spectrometry; Evaporation; Analytical Chemistry (journal); Electrostatics; Molecular dynamics; Chromatography; Chemical physics; Computational chemistry; Physical chemistry; Organic chemistry; Thermodynamics","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":["insufficient_payload"],"consensus_categories":[],"category_scores_codex":[0.0001394791,0.0001726323,0.0002371926,0.00003068943,0.00005632704,0.00002885689,0.000324763,0.0001677072,0.001089006],"category_scores_gemma":[0.0001164323,0.0001443576,0.0001179038,0.0006425297,0.00007036797,0.0001072541,0.00004923476,0.0004397324,0.000009425215],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0001459472,"about_ca_system_score_gemma":0.00005489603,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00001246835,"about_ca_topic_score_gemma":0.000001989709,"domain_scores_codex":[0.9986216,0.000009389606,0.000472953,0.0002952634,0.0003275266,0.000273263],"domain_scores_gemma":[0.999209,0.00004463586,0.0001878521,0.0003827841,0.0000697893,0.0001059471],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00003124616,0.00008279653,0.0001926868,0.000201368,0.00001103887,0.000002292078,0.00003718402,0.000348364,0.99673,0.001939331,0.0002499926,0.0001737011],"study_design_scores_gemma":[0.0001462059,0.00001736763,0.00001166677,0.00001359417,0.00002261322,0.000004519948,0.00003139753,0.3071115,0.6854898,0.006887973,0.0001541251,0.0001092747],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.5040656,0.0001508367,0.3610924,0.01042914,0.000006856635,0.0005471041,0.00007201288,0.0003444579,0.1232916],"genre_scores_gemma":[0.9963109,0.00002745881,0.002976947,0.0001160011,0.000107455,0.00007189666,0.0000936443,0.00001883102,0.0002768729],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.4922453,"threshold_uncertainty_score":0.9998241,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01640057571713101,"score_gpt":0.2525452956976313,"score_spread":0.2361447199805003,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}