{"id":"W3093892917","doi":"10.1039/d1ee01037a","title":"Coulombically-stabilized oxygen hole polarons enable fully reversible oxygen redox","year":2021,"lang":"en","type":"article","venue":"Energy & Environmental Science","topic":"Electrocatalysts for Energy Conversion","field":"Energy","cited_by":59,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Waterloo","funders":"Division of Materials Sciences and Engineering; SLAC National Accelerator Laboratory; Natural Sciences and Engineering Research Council of Canada; Office of Science; Canada Research Chairs; Basic Energy Sciences; Division of Electrical, Communications and Cyber Systems; National Energy Research Scientific Computing Center; U.S. Department of Energy; National Science Foundation","keywords":"Redox; Faraday efficiency; Covalent bond; Oxygen; Polaron; Electrochemistry; Oxide","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001155884,0.000318474,0.0001754084,0.0001211941,0.0002013873,0.000564753,0.0004111869,0.0003904523,0.004640841],"category_scores_gemma":[0.0003947039,0.0001161134,0.00008554515,0.0001365153,0.0002607099,0.0006013345,0.0005745583,0.0005448288,0.0006167699],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.000213101,"about_ca_system_score_gemma":0.0001630802,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0003721708,"about_ca_topic_score_gemma":0.001512026,"domain_scores_codex":[0.9999145,0.000006025719,0.000003321301,0.0000176171,0.00003161463,0.00002695502],"domain_scores_gemma":[0.9999127,0.00002394482,0.00001829442,0.00001111323,0.00002006184,0.00001388566],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00009168493,0.00005065897,0.0002619231,0.0001562676,0.00001301919,0.0001321844,0.00004373036,0.0003884814,0.9733145,0.007234727,0.001814161,0.01649872],"study_design_scores_gemma":[0.00002209473,0.0002615788,0.0007266417,0.00001731099,0.0000125097,0.000179866,0.0001133932,0.003724789,0.9807943,0.001809405,0.01232211,0.00001602367],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9302488,0.002175845,0.03261678,0.0006828228,0.0006725903,0.0000791562,0.0005299191,0.0006166025,0.03237753],"genre_scores_gemma":[0.993172,0.0004191127,0.002675062,0.0001209194,0.00001935754,0.00001359004,0.0001894326,0.00003794742,0.003352622],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.004640841,"threshold_uncertainty_score":0.01552516,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.005745249710832376,"score_gpt":0.1992616039170674,"score_spread":0.193516354206235,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}