{"id":"W3128945229","doi":"10.1021/acsenergylett.0c02401","title":"Self-Cleaning CO<sub>2</sub> Reduction Systems: Unsteady Electrochemical Forcing Enables Stability","year":2021,"lang":"en","type":"article","venue":"ACS Energy Letters","topic":"CO2 Reduction Techniques and Catalysts","field":"Energy","cited_by":380,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Toronto","funders":"Natural Resources Canada; Natural Sciences and Engineering Research Council of Canada; Total; University of Toronto; Canada Research Chairs; Government of Ontario","keywords":"Electrochemistry; Electrolysis; Cathode; Gas diffusion electrode; Chemical engineering; Electrode; Selectivity; Copper; Materials science; Gaseous diffusion; Catalysis; Inorganic chemistry; Membrane electrode assembly; Chemistry; Metallurgy; Anode; Electrolyte","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0002093928,0.00032807,0.0003237333,0.0001712626,0.0002666573,0.0005245456,0.0005282779,0.0004331081,0.0008710477],"category_scores_gemma":[0.0005115519,0.0002067307,0.0001426273,0.0001772812,0.0003750976,0.0006549312,0.000389613,0.0005477844,0.0004599719],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0004823239,"about_ca_system_score_gemma":0.0001955667,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0006994225,"about_ca_topic_score_gemma":0.001971636,"domain_scores_codex":[0.9997589,0.00002200974,0.00001642567,0.00007093557,0.00008544427,0.00004628998],"domain_scores_gemma":[0.9997645,0.00005206363,0.00005707851,0.0000552697,0.00005278677,0.00001824206],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00003758864,0.00001090051,0.0001448141,0.0000339507,0.000004962535,0.00003133677,0.00002405737,0.00008252267,0.9961942,0.000208635,0.0001159992,0.00311089],"study_design_scores_gemma":[0.00000250167,0.00002307712,0.0003430732,8.657142e-7,0.000002147375,0.00004640003,0.000007178765,0.0008399113,0.9976341,0.00002874813,0.001069502,0.000002599582],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.955608,0.00255419,0.03693808,0.0005397426,0.0001013631,0.0000536388,0.000171582,0.000562967,0.003470404],"genre_scores_gemma":[0.9852251,0.0006163234,0.01165844,0.00008147264,0.00002732036,0.00003715327,0.0001487979,0.00007060592,0.002134586],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0008710477,"threshold_uncertainty_score":0.003499508,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.009015416215025225,"score_gpt":0.2094779326739819,"score_spread":0.2004625164589567,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}