{"id":"W3131380119","doi":"10.1038/s41467-021-21401-2","title":"Phase-enabled metal-organic framework homojunction for highly selective CO2 photoreduction","year":2021,"lang":"en","type":"article","venue":"Nature Communications","topic":"Metal-Organic Frameworks: Synthesis and Applications","field":"Chemistry","cited_by":105,"is_retracted":false,"has_abstract":true,"ca_institutions":"McGill University; Canadian Light Source (Canada); Institut National de la Recherche Scientifique","funders":"Natural Sciences and Engineering Research Council of Canada; Argonne National Laboratory; Shanghai Jiao Tong University; Canadian Network for Research and Innovation in Machining Technology, Natural Sciences and Engineering Research Council of Canada; Office of Science; Canada Research Chairs; Compute Canada; Fonds de recherche du Québec – Nature et technologies; Canadian Light Source; U.S. Department of Energy","keywords":"Homojunction; Materials science; Nanotechnology; Metal-organic framework; Photocatalysis; Surface photovoltage; Charge carrier; Electrochemical reduction of carbon dioxide; Chemical engineering; Optoelectronics; Doping; Chemistry; Catalysis; Organic chemistry; Spectroscopy","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.00008170307,0.0002945581,0.0001780809,0.0002274876,0.0001488203,0.0003392127,0.0005222908,0.0003230069,0.0007344969],"category_scores_gemma":[0.0001018203,0.0001690328,0.0001490106,0.000208966,0.0001409694,0.0003486006,0.0002447092,0.0003052447,0.0002277419],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0003376765,"about_ca_system_score_gemma":0.000164577,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0006256099,"about_ca_topic_score_gemma":0.002643527,"domain_scores_codex":[0.999909,0.000005380907,0.000004364861,0.00002707839,0.00002489445,0.00002912682],"domain_scores_gemma":[0.9999692,0.000005760206,0.000007642394,0.000005213897,0.000006057612,0.000006079576],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00001769789,0.00002516788,0.00004667025,0.00007292625,0.000008244234,0.00006989986,0.00001482915,0.0003621192,0.9942223,0.0007366231,0.0002224122,0.004201123],"study_design_scores_gemma":[0.000007609382,0.0000858835,0.0005410262,0.000003126573,0.000007521713,0.0001141683,0.00001098501,0.002762086,0.9932902,0.00009195616,0.003077417,0.000007981359],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9653478,0.004560652,0.0204478,0.0001508077,0.0002538542,0.00004933006,0.0005967239,0.001031004,0.007562085],"genre_scores_gemma":[0.9886082,0.00104895,0.008043626,0.00003887383,0.00001680947,0.00001682732,0.0001756331,0.00003429661,0.002016639],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0007344969,"threshold_uncertainty_score":0.002457201,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01884833833368441,"score_gpt":0.2953646619566165,"score_spread":0.276516323622932,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}