{"id":"W3156138561","doi":"10.1021/jacs.1c00384","title":"Stabilizing Highly Active Ru Sites by Suppressing Lattice Oxygen Participation in Acidic Water Oxidation","year":2021,"lang":"en","type":"article","venue":"Journal of the American Chemical Society","topic":"Electrocatalysts for Energy Conversion","field":"Energy","cited_by":548,"is_retracted":false,"has_abstract":true,"ca_institutions":"Canadian Light Source (Canada); Queen's University; Canada Research Chairs; University of Toronto","funders":"Division of Chemical, Bioengineering, Environmental, and Transport Systems; Beijing Synchrotron Radiation Facility; Natural Sciences and Engineering Research Council of Canada; Office of Science; Ministry of Science and Technology of the People's Republic of China; Northwestern Polytechnical University; U.S. Department of Energy; California Institute of Technology; Salt Science Research Foundation; Canadian Institute for Advanced Research; E-Institutes of Shanghai Municipal Education Commission; Shanghai Municipal Education Commission; National Natural Science Foundation of China; Northwestern University; Science and Technology Commission of Shanghai Municipality; National Science Foundation","keywords":"Chemistry; Overpotential; Oxygen evolution; Water splitting; Catalysis; Inorganic chemistry; Electrolyte; Electrochemistry; Physical chemistry; Electrode; Photocatalysis","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0002760807,0.000123267,0.0002648177,0.00001861731,0.00007969254,0.00003606694,0.0002261366,0.00006188436,0.00004269968],"category_scores_gemma":[0.0002105012,0.00008183756,0.0002662123,0.0003638053,0.0001729674,0.0003114846,0.0001170208,0.0003739684,0.000003796091],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0005753594,"about_ca_system_score_gemma":0.00007191349,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0001814469,"about_ca_topic_score_gemma":0.00002627699,"domain_scores_codex":[0.9986034,0.0001534542,0.0003663932,0.0001622259,0.00042113,0.0002934006],"domain_scores_gemma":[0.9990088,0.0001445288,0.0003877202,0.0001821547,0.0002068936,0.0000699429],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00006068706,0.00009106882,0.001118124,0.0000084272,0.00007845531,0.000002390544,0.001060773,0.0002439441,0.9945732,0.00001498559,0.0009803631,0.001767581],"study_design_scores_gemma":[0.0003779484,0.00002867805,0.001169218,0.00002701239,0.00006637825,0.00001205106,0.0008919559,0.0004213213,0.9950784,0.0002452259,0.001573282,0.0001084768],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9966752,0.00009072619,0.00008198772,0.002946495,0.0000557311,0.00002655081,8.218817e-7,0.00001206302,0.0001104594],"genre_scores_gemma":[0.9983295,0.00004761843,0.0008464215,0.000570862,0.0001045609,0.000002256063,0.0000245414,0.00001901716,0.00005521367],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.002375633,"threshold_uncertainty_score":0.3337239,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01029295483206976,"score_gpt":0.2544510945883038,"score_spread":0.2441581397562341,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}