{"id":"W4200604942","doi":"10.1002/ange.202111351","title":"Electron Localization and Lattice Strain Induced by Surface Lithium Doping Enable Ampere‐Level Electrosynthesis of Formate from CO<sub>2</sub>","year":2021,"lang":"en","type":"article","venue":"Angewandte Chemie","topic":"CO2 Reduction Techniques and Catalysts","field":"Energy","cited_by":32,"is_retracted":false,"has_abstract":true,"ca_institutions":"Western University","funders":"National Key Research and Development Program of China; Science and Technology Commission of Shanghai Municipality; Shanghai Municipal Education Commission; National Natural Science Foundation of China","keywords":"Formate; Electrosynthesis; Electrochemistry; Electrocatalyst; Catalysis; Faraday efficiency; Chemistry; Doping; Inorganic chemistry; Materials science; Chemical engineering; Nanotechnology; Physical chemistry; Electrode; Organic chemistry; Optoelectronics","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0000675132,0.0002385297,0.000112083,0.0001076752,0.0000938946,0.0002783577,0.000254128,0.0001775009,0.0008267104],"category_scores_gemma":[0.0001467838,0.000118156,0.0001003983,0.00009073514,0.0002864939,0.0002885998,0.0002011669,0.000275915,0.0002711417],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002794274,"about_ca_system_score_gemma":0.0001308937,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0003905063,"about_ca_topic_score_gemma":0.000879703,"domain_scores_codex":[0.9999479,0.000005130085,0.000004126867,0.00001083895,0.00002157636,0.00001043208],"domain_scores_gemma":[0.9999477,0.00001085066,0.00001614019,0.000007179169,0.00001271867,0.000005483491],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0000360713,0.00001205988,0.0001769931,0.00002688454,0.000002861281,0.00003962708,0.000012156,0.0002632012,0.9957823,0.0004623919,0.00005858899,0.003126954],"study_design_scores_gemma":[0.000003475709,0.00003133993,0.0002576671,0.000001107622,0.00000256628,0.00003951264,0.000006857447,0.002019744,0.9969829,0.00004508993,0.0006076749,0.000002054468],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9777946,0.0004706425,0.017236,0.0001577906,0.00006113095,0.00001429311,0.0000606859,0.0002651379,0.003939637],"genre_scores_gemma":[0.9947773,0.0001679478,0.003409185,0.00002329085,0.000005917234,0.000005896847,0.00004750949,0.00001913648,0.00154378],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0008267104,"threshold_uncertainty_score":0.002765656,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01733751275890611,"score_gpt":0.2400348008768348,"score_spread":0.2226972881179287,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}