{"id":"W4205352653","doi":"10.1021/acscatal.1c04407","title":"Au(001) Thin Films: Impact of Structure and Mosaicity on the Oxygen Reduction Reaction in Alkaline Medium","year":2022,"lang":"en","type":"article","venue":"ACS Catalysis","topic":"Electrocatalysts for Energy Conversion","field":"Energy","cited_by":3,"is_retracted":false,"has_abstract":true,"ca_institutions":"Université de Montréal; Collège de Maisonneuve; Institut National de la Recherche Scientifique","funders":"Fonds de recherche du Québec – Nature et technologies; Natural Sciences and Engineering Research Council of Canada","keywords":"Cyclic voltammetry; Thin film; Epitaxy; Analytical Chemistry (journal); Materials science; Mosaicity; Substrate (aquarium); Underpotential deposition; Electrode; Electrolyte; Pulsed laser deposition; Single crystal; Chemistry; Inorganic chemistry; Electrochemistry; Crystallography; Nanotechnology; Physical chemistry","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0004719933,0.0001744545,0.0002486943,0.00028596,0.0002145185,0.00001063248,0.0002487129,0.00008435814,0.0003502061],"category_scores_gemma":[0.0001231922,0.0001296588,0.0001110523,0.0009191364,0.00006389737,0.0001725792,0.0001423961,0.0003664838,0.00000495224],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0006366764,"about_ca_system_score_gemma":0.0001000857,"about_ca_topic_candidate":true,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.04523629,"about_ca_topic_score_gemma":0.003027182,"domain_scores_codex":[0.9985052,0.0001835293,0.0002837433,0.0003223117,0.0004728753,0.0002322793],"domain_scores_gemma":[0.999069,0.00009154609,0.0002178375,0.0005107192,0.00006235115,0.0000485088],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0002915762,0.0001296219,0.0007986012,0.00001202631,0.0003128686,0.000005679281,0.00160694,0.03093571,0.9600714,0.001146634,0.002006154,0.002682782],"study_design_scores_gemma":[0.001496713,0.0007487025,0.02681737,0.0000238806,0.0003853429,0.0001194735,0.002639128,0.004566818,0.9554129,0.002918334,0.004326206,0.0005451764],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9986878,0.00006078443,0.000001598348,0.0005272673,0.0001239047,0.00009870946,0.00002488199,0.00003296537,0.0004420803],"genre_scores_gemma":[0.9983686,0.00003323401,0.00001491529,0.00005684432,0.00006691924,0.00002197296,0.001047275,0.00002315898,0.0003671232],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.04220911,"threshold_uncertainty_score":0.9611216,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.00789818219603754,"score_gpt":0.22736446641702,"score_spread":0.2194662842209824,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}