{"id":"W4205364322","doi":"10.1002/smll.202106614","title":"Atomically Defined Undercoordinated Copper Active Sites over Nitrogen‐Doped Carbon for Aerobic Oxidation of Alcohols","year":2022,"lang":"en","type":"article","venue":"Small","topic":"Oxidative Organic Chemistry Reactions","field":"Chemistry","cited_by":27,"is_retracted":false,"has_abstract":true,"ca_institutions":"Queen's University","funders":"China Postdoctoral Science Foundation","keywords":"Catalysis; Alcohol oxidation; Copper; Cinnamyl alcohol; Oxidation state; Carbon fibers; Substrate (aquarium); Heterogeneous catalysis","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0000977428,0.0002945491,0.000175931,0.000220877,0.0001499014,0.0002740462,0.0004810665,0.0002535218,0.000569852],"category_scores_gemma":[0.0001618556,0.000131275,0.00009116576,0.0001898016,0.0002635671,0.000210042,0.0002355889,0.0002713421,0.0001429652],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0004364736,"about_ca_system_score_gemma":0.0001992595,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.001617679,"about_ca_topic_score_gemma":0.003609256,"domain_scores_codex":[0.9998716,0.00001131616,0.000007886566,0.00002966427,0.00005276238,0.00002675594],"domain_scores_gemma":[0.9999354,0.000009680124,0.00001656901,0.0000105464,0.00001462977,0.000013118],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00008657678,0.0000333077,0.0003302614,0.0001028288,0.00001230669,0.0001557434,0.00002915719,0.0007371205,0.9932186,0.0006517193,0.0002832442,0.004359139],"study_design_scores_gemma":[0.00001789462,0.0001495461,0.001184182,0.000007160366,0.00001180454,0.0001188944,0.00002623768,0.004897782,0.9902359,0.00007454814,0.003264638,0.00001139665],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9924389,0.0008875491,0.002352804,0.00007373912,0.00004815726,0.00001665204,0.0001032788,0.00008176792,0.003997187],"genre_scores_gemma":[0.9980495,0.0002223654,0.001138892,0.00001037109,0.000005344239,0.000006123263,0.00005452954,0.000009220333,0.0005036775],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.001617679,"threshold_uncertainty_score":0.003216505,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.0262946015706648,"score_gpt":0.2511246033608513,"score_spread":0.2248300017901865,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}