{"id":"W4205808442","doi":"10.1021/acsaem.1c02522","title":"Impact of Nickel Content on the Structure and Electrochemical CO<sub>2</sub> Reduction Performance of Nickel–Nitrogen–Carbon Catalysts Derived from Zeolitic Imidazolate Frameworks","year":2022,"lang":"en","type":"article","venue":"ACS Applied Energy Materials","topic":"CO2 Reduction Techniques and Catalysts","field":"Energy","cited_by":28,"is_retracted":false,"has_abstract":true,"ca_institutions":"McMaster University","funders":"National Research Council Canada; McMaster University","keywords":"Catalysis; Nickel; Zeolitic imidazolate framework; Electrochemistry; Faraday efficiency; Materials science; Selectivity; Imidazolate; Carbon fibers; Chemical engineering; Inorganic chemistry; Transition metal; Nitrogen; Pyrolysis; Metal-organic framework; Chemistry; Electrode; Organic chemistry; Adsorption; Metallurgy; Composite number","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001383009,0.0003065133,0.00017908,0.0001638483,0.000152701,0.0004726028,0.0004471387,0.000287999,0.0007423285],"category_scores_gemma":[0.0004094252,0.0002351555,0.0001086919,0.0001390536,0.0001821398,0.0002851635,0.0001279008,0.0002494855,0.0002317357],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0004356874,"about_ca_system_score_gemma":0.0001594647,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00175462,"about_ca_topic_score_gemma":0.003736714,"domain_scores_codex":[0.9998263,0.00001471428,0.00001529289,0.00003824347,0.00006195238,0.00004356559],"domain_scores_gemma":[0.9998605,0.00003835685,0.00003968773,0.00001213091,0.00003527252,0.00001400986],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.000175453,0.00002513685,0.000517928,0.00003693948,0.000007692877,0.00005626365,0.00002267599,0.0002274199,0.9970751,0.00008455772,0.00004381608,0.00172701],"study_design_scores_gemma":[0.000003663614,0.00005699066,0.001199846,0.000001651241,0.000007812021,0.00002524039,0.00001075281,0.001056783,0.997395,0.000006910916,0.0002325934,0.000002591285],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9982973,0.0002803537,0.0002686877,0.00002275217,0.000006108357,0.000005749631,0.00008544084,0.00002842706,0.001005251],"genre_scores_gemma":[0.9990902,0.0001419395,0.0003398009,0.00000882427,0.000002338221,0.000005923057,0.00008937697,0.00001035558,0.0003112107],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.00175462,"threshold_uncertainty_score":0.003488839,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.008779596020110594,"score_gpt":0.2156850844516375,"score_spread":0.206905488431527,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}