{"id":"W4213092750","doi":"10.26434/chemrxiv-2022-p5fwp","title":"Water Dipole Populations in the Electrical Double Layer and Their Contributions to the Total Interfacial Potential at Different Surface Charge Densities","year":2022,"lang":"en","type":"preprint","venue":"ChemRxiv","topic":"Spectroscopy and Quantum Chemical Studies","field":"Physics and Astronomy","cited_by":2,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Alberta","funders":"","keywords":"Dipole; Aqueous solution; Chemistry; Chemical physics; Molecule; Double layer (biology); Electric potential; Electrolyte; Molecular physics; Layer (electronics); Analytical Chemistry (journal); Physical chemistry; Physics; Organic chemistry; Voltage","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0002052696,0.0003275481,0.0001522064,0.0006191478,0.0001307878,0.0003139865,0.0002475589,0.0002272417,0.001393122],"category_scores_gemma":[0.0004934286,0.0001670007,0.0001401577,0.0002723914,0.0004021899,0.0005869681,0.0004228188,0.0002918741,0.0001695072],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.000154029,"about_ca_system_score_gemma":0.00008464089,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0002882501,"about_ca_topic_score_gemma":0.000249431,"domain_scores_codex":[0.9999211,0.000007472991,0.000002881438,0.00002562717,0.00002461279,0.00001836114],"domain_scores_gemma":[0.9998726,0.00005323582,0.00002343226,0.00000999973,0.00002461131,0.00001620598],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"simulation_or_modeling","study_design_scores_codex":[0.00009136485,0.0000226597,0.003365816,0.00007956583,0.0000216778,0.00009247543,0.0001499824,0.002483046,0.9849463,0.00123549,0.00006521374,0.007446411],"study_design_scores_gemma":[0.00002922699,0.000214045,0.0456811,0.00001805248,0.00005295414,0.0003097417,0.0003888479,0.0585539,0.8899176,0.003514422,0.001279255,0.00004078837],"study_design_candidate":"simulation_or_modeling","study_design_consensus":null,"genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9903556,0.0003675955,0.007675148,0.00004125834,0.000008303087,0.000007904725,0.0001035399,0.00006730233,0.001373402],"genre_scores_gemma":[0.9982628,0.0001849906,0.001001153,0.00001134827,0.000003462053,0.000009563732,0.00008243827,0.0000128588,0.0004313671],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.001393122,"threshold_uncertainty_score":0.004660428,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.02463136002452772,"score_gpt":0.2852846923972318,"score_spread":0.260653332372704,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}