{"id":"W4283020322","doi":"10.1038/s41557-022-00967-4","title":"In situ electrochemical recomposition of decomposed redox-active species in aqueous organic flow batteries","year":2022,"lang":"en","type":"article","venue":"Nature Chemistry","topic":"Advanced battery technologies research","field":"Engineering","cited_by":145,"is_retracted":false,"has_abstract":false,"ca_institutions":"Concordia University","funders":"Pacific Northwest National Laboratory; Division of Chemical, Bioengineering, Environmental, and Transport Systems; Massachusetts Clean Energy Center; Engineering and Physical Sciences Research Council; U.S. Department of Energy; Science and Technology Facilities Council; National Science Foundation","keywords":"Chemistry; Redox; Electrochemistry; Aqueous solution; Electrolyte; Electron transfer; Decomposition; Supporting electrolyte; Combinatorial chemistry; Inorganic chemistry; Photochemistry; Organic chemistry; Electrode; Physical chemistry","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001953418,0.0002374027,0.0001759847,0.0001907799,0.0001382238,0.0004015354,0.0003616062,0.0003366144,0.001550963],"category_scores_gemma":[0.0002670018,0.0001467049,0.0001243979,0.0001654206,0.0002331201,0.000384492,0.0001396804,0.0003385162,0.0001558064],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.00021336,"about_ca_system_score_gemma":0.0001310178,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0005568331,"about_ca_topic_score_gemma":0.0008724898,"domain_scores_codex":[0.999893,0.00001235392,0.000005994821,0.0000277919,0.00003106107,0.00002983539],"domain_scores_gemma":[0.9999374,0.00002098454,0.00001360424,0.000007133002,0.00001325916,0.000007680054],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0001199929,0.00002397776,0.000091577,0.00005103638,0.000004990871,0.00004478871,0.00004088732,0.0001332234,0.9965432,0.0001118259,0.00003787352,0.002796566],"study_design_scores_gemma":[0.000005722914,0.00007884688,0.0002760569,0.000001790293,0.000003492756,0.00002276953,0.00001661057,0.0006221125,0.9985325,0.00001502271,0.0004232272,0.000001832715],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9964975,0.0005061755,0.001714514,0.00004160338,0.0000293862,0.000009931193,0.0000876146,0.00003331112,0.001080182],"genre_scores_gemma":[0.997118,0.0002672358,0.001050077,0.00001901168,0.000008671024,0.000004294605,0.00006492652,0.00001204036,0.00145576],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.001550963,"threshold_uncertainty_score":0.005188525,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.003871645620480809,"score_gpt":0.2291596470355574,"score_spread":0.2252880014150766,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}