{"id":"W4310009701","doi":"10.1038/s41467-022-35046-2","title":"Energy cascades in donor-acceptor exciton-polaritons observed by ultrafast two-dimensional white-light spectroscopy","year":2022,"lang":"en","type":"article","venue":"Nature Communications","topic":"Strong Light-Matter Interactions","field":"Physics and Astronomy","cited_by":72,"is_retracted":false,"has_abstract":true,"ca_institutions":"","funders":"Air Force Office of Scientific Research; Polytechnique Montréal; U.S. Department of Defense","keywords":"Exciton; Polariton; Spectroscopy; Intermolecular force; Acceptor; Molecular physics; Physics; Atomic physics; Ultrashort pulse; Chemical physics; Materials science; Optoelectronics; Condensed matter physics; Optics; Quantum mechanics; Molecule; Laser","routes":{"ca_aff":false,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":true},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001261417,0.0001877715,0.0001149818,0.0001839662,0.0002524193,0.0003306047,0.0002394496,0.0002627596,0.0008969479],"category_scores_gemma":[0.000348563,0.0001742502,0.0001486167,0.0001347484,0.0004494452,0.0004936946,0.000323841,0.0004473802,0.00007912552],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0004005347,"about_ca_system_score_gemma":0.0001105511,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0004829627,"about_ca_topic_score_gemma":0.0003841346,"domain_scores_codex":[0.9999374,0.000009133381,0.000002185301,0.0000127518,0.00002492537,0.00001363297],"domain_scores_gemma":[0.9998654,0.00006697022,0.00002934817,0.00001184772,0.00001099879,0.00001545008],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.000126945,0.0001182068,0.002552106,0.00003143801,0.00001616078,0.0002517566,0.0002332903,0.01241909,0.9744278,0.007261458,0.00006809772,0.002493725],"study_design_scores_gemma":[0.00005233533,0.0002158922,0.01016615,0.00000900252,0.00001670281,0.0002285996,0.0001561883,0.2514865,0.7327068,0.004319275,0.0006106009,0.00003199274],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9978942,0.00001475962,0.001446413,0.00001414768,0.000001663019,0.000003153576,0.000009428297,0.00001712327,0.0005991348],"genre_scores_gemma":[0.9987211,0.00001663078,0.001019523,0.000004629119,5.92256e-7,0.00000517668,0.000008087698,0.000004669761,0.0002197099],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0008969479,"threshold_uncertainty_score":0.003000617,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01397504355870477,"score_gpt":0.2804239646135487,"score_spread":0.266448921054844,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}