{"id":"W4310009701","doi":"10.1038/s41467-022-35046-2","title":"Energy cascades in donor-acceptor exciton-polaritons observed by ultrafast two-dimensional white-light spectroscopy","year":2022,"lang":"en","type":"article","venue":"Nature Communications","topic":"Strong Light-Matter Interactions","field":"Physics and Astronomy","cited_by":72,"is_retracted":false,"has_abstract":true,"ca_institutions":"","funders":"Air Force Office of Scientific Research; Polytechnique Montréal; U.S. Department of Defense","keywords":"Exciton; Polariton; Spectroscopy; Intermolecular force; Acceptor; Molecular physics; Physics; Atomic physics; Ultrashort pulse; Chemical physics; Materials science; Optoelectronics; Condensed matter physics; Optics; Quantum mechanics; Molecule; Laser","routes":{"ca_aff":false,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":true},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":["metaepi_narrow","insufficient_payload"],"consensus_categories":[],"category_scores_codex":[0.0001349064,0.0002512536,0.0002537327,0.0001942735,0.0008902395,0.00009681059,0.001553874,0.00008571721,0.002663056],"category_scores_gemma":[0.000009151447,0.0002783052,0.0001647059,0.0005974653,0.00008086135,0.0002578649,0.0007051683,0.002054453,0.00003280761],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002527322,"about_ca_system_score_gemma":0.0001223794,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.001304924,"about_ca_topic_score_gemma":0.0009653887,"domain_scores_codex":[0.9982201,0.0003476463,0.0004027296,0.0003637758,0.0002905428,0.0003751842],"domain_scores_gemma":[0.9976594,0.0003202709,0.0001803377,0.001648002,0.00008347407,0.0001085149],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"not_applicable","study_design_scores_codex":[0.0000482999,0.001970797,0.1479651,0.0000042786,0.0002582642,0.000002603872,0.0008393694,0.0006967542,0.5583891,0.01841047,0.271026,0.0003890471],"study_design_scores_gemma":[0.002310854,0.0001207308,0.02382702,0.00004599001,0.0001119745,0.0000260733,0.002398299,0.0007221422,0.2655044,0.00252913,0.7011987,0.001204684],"study_design_candidate":"not_applicable","study_design_consensus":null,"genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.8852394,0.003832638,0.0002956277,0.05357802,0.002523092,0.0007977674,0.003218777,0.0003243855,0.05019031],"genre_scores_gemma":[0.9926611,0.000001374214,0.002866698,0.0006049777,0.0001937254,0.0004399106,0.001787395,0.00004453717,0.001400308],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.4301727,"threshold_uncertainty_score":0.9999669,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01397504355870477,"score_gpt":0.2804239646135487,"score_spread":0.266448921054844,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}