{"id":"W4388626081","doi":"10.1016/j.cej.2023.147359","title":"Crossover, volatilization, and adsorption of ammonium ions in a proton-exchange membrane electrolyzer in relation to electrochemical ammonia production","year":2023,"lang":"en","type":"article","venue":"Chemical Engineering Journal","topic":"Ammonia Synthesis and Nitrogen Reduction","field":"Chemical Engineering","cited_by":10,"is_retracted":false,"has_abstract":false,"ca_institutions":"University of British Columbia","funders":"National Research Council Canada; University of British Columbia; National Research Council","keywords":"Chemistry; Inorganic chemistry; Electrolysis; Electrolyte; Electrochemistry; Nafion; Ammonium; Ammonia; Adsorption; Organic chemistry; Electrode","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0003765518,0.0001984819,0.0002971198,0.0005108465,0.00002674435,0.00002462569,0.0001024217,0.0001961629,0.00001041681],"category_scores_gemma":[0.0006999176,0.0002086763,0.00006379809,0.001230302,0.00002300749,0.0002248817,0.00004027417,0.0005582215,0.000006181722],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002668474,"about_ca_system_score_gemma":0.00003249041,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00001138065,"about_ca_topic_score_gemma":0.000002592066,"domain_scores_codex":[0.9984413,0.00001785461,0.0005606188,0.0002949536,0.0002629468,0.0004223616],"domain_scores_gemma":[0.9994832,0.00006289362,0.00009777626,0.0001327845,0.00008229718,0.0001410334],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0001908824,0.00005350863,0.0007939715,0.0001660389,0.00001413484,0.000002476435,0.0002901403,0.01357733,0.9842571,0.0001097734,0.00002530755,0.0005193409],"study_design_scores_gemma":[0.000478524,0.00002769408,0.002064842,0.0002066559,0.00001114572,0.00006722103,0.00001737275,0.132942,0.863795,0.00005772434,0.0001508391,0.000180965],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9920894,0.0002186535,0.006830354,0.0002785452,0.0001127336,0.0003481813,0.000001517839,0.0001079713,0.00001263481],"genre_scores_gemma":[0.9966348,0.0001851716,0.002738385,0.000006089212,0.0002279222,0.0001028285,0.00001603636,0.00004541984,0.00004329293],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.1204621,"threshold_uncertainty_score":0.850957,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.008377918601328227,"score_gpt":0.2216668421831369,"score_spread":0.2132889235818086,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}