{"id":"W4389067883","doi":"10.1016/j.jpowsour.2023.233882","title":"Imaging the space-resolved chemical heterogeneity of degraded graphite anode through scanning transmission X-ray microscope","year":2023,"lang":"en","type":"article","venue":"Journal of Power Sources","topic":"Advancements in Battery Materials","field":"Engineering","cited_by":10,"is_retracted":false,"has_abstract":false,"ca_institutions":"Canadian Light Source (Canada); University of Saskatchewan","funders":"Government of Saskatchewan; Fundamental Research Funds for the Central Universities; Natural Sciences and Engineering Research Council of Canada; Science, Technology and Innovation Commission of Shenzhen Municipality; National University's Basic Research Foundation of China; National Natural Science Foundation of China; Canada Foundation for Innovation; Canadian Institutes of Health Research; National Research Council; University of Saskatchewan","keywords":"Chemical imaging; Anode; Chemical state; X-ray photoelectron spectroscopy; Graphite; Analytical Chemistry (journal); XANES; Microscope; Electrolyte; Transmission electron microscopy; Chemistry; Materials science; Synchrotron; Chemical engineering; Electrode; Spectroscopy; Nanotechnology; Optics; Composite material; Physics; Organic chemistry","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0003968733,0.0001830633,0.0003333342,0.0001219736,0.00007474858,0.00004552774,0.0003640735,0.00004918129,0.00005690068],"category_scores_gemma":[0.00002871603,0.0001264052,0.0001365801,0.0002838021,0.0001166131,0.0002616822,0.00004891741,0.0002033737,0.000005067989],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.00003202691,"about_ca_system_score_gemma":0.00001151161,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.000002538591,"about_ca_topic_score_gemma":1.63707e-7,"domain_scores_codex":[0.9986451,0.00005605396,0.0005788906,0.000112395,0.0003183717,0.0002891923],"domain_scores_gemma":[0.9993666,0.00008238008,0.0002410075,0.0001915496,0.00006022608,0.00005818288],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00003813773,0.00001585033,0.002984793,0.0000527266,0.00008024518,0.00001647236,0.002455331,0.008286651,0.9843383,0.000004044645,0.001266038,0.0004613826],"study_design_scores_gemma":[0.0005825256,0.00003750463,0.003932004,0.0003156936,0.00005393923,0.000043174,0.0006355898,0.0003836483,0.9818061,0.0002474316,0.01177709,0.0001853097],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9826792,0.001770006,0.01420753,0.0003401348,0.0007724879,0.00008301474,0.000007966644,0.00006708632,0.00007257762],"genre_scores_gemma":[0.9955302,0.000160669,0.004054289,0.00007312731,0.0001194877,0.00000201779,0.000001580812,0.00004324652,0.00001537392],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.01285101,"threshold_uncertainty_score":0.5154654,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01467319895509494,"score_gpt":0.2607715363303618,"score_spread":0.2460983373752668,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}