{"id":"W4389358776","doi":"10.1021/jacs.3c07668","title":"Visualizing the Birth and Monitoring the Life of a Bimetallic Methanation Catalyst","year":2023,"lang":"en","type":"article","venue":"Journal of the American Chemical Society","topic":"Catalytic Processes in Materials Science","field":"Materials Science","cited_by":28,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Toronto; Queen's University","funders":"Zhejiang University; Natural Sciences and Engineering Research Council of Canada; National Natural Science Foundation of China; University of Toronto; Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering","keywords":"Methanation; Bimetallic strip; Catalysis; Chemistry; Nanoparticle; Ruthenium; Chemical engineering; X-ray absorption spectroscopy; Photochemistry; Inorganic chemistry; Absorption spectroscopy; Organic chemistry","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.002310622,0.0000987645,0.0002613847,0.00001925263,0.0001994458,0.00009169972,0.001035403,0.00002317854,0.000008855984],"category_scores_gemma":[0.001099601,0.00004327485,0.0001866291,0.0009581935,0.001204051,0.0001590113,0.0004485877,0.0001737004,0.00000430985],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0000520474,"about_ca_system_score_gemma":0.0001108741,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00008584207,"about_ca_topic_score_gemma":4.212798e-7,"domain_scores_codex":[0.9985317,0.00009204954,0.000409148,0.0001323439,0.0006303025,0.0002044676],"domain_scores_gemma":[0.997969,0.0005680242,0.0009862784,0.0002759214,0.0001400451,0.00006073524],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00001091208,0.000009604164,0.0003671498,0.00002292897,0.00002369879,2.902731e-7,0.001081928,0.00004908329,0.9977196,0.0000320894,0.0003770798,0.0003056097],"study_design_scores_gemma":[0.00009582854,0.00002143647,0.002452671,0.00003817726,0.00005908603,0.00003004814,0.002637648,0.0003353517,0.9934728,0.0005415392,0.0002535405,0.00006187995],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.996379,0.000226697,0.0001363997,0.002791131,0.000365692,0.00006813434,0.000005602367,0.0000150477,0.000012269],"genre_scores_gemma":[0.9985444,0.0001802092,0.0007442614,0.0002384909,0.0002621101,0.000003367045,1.760207e-7,0.000009278986,0.00001770755],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.004246832,"threshold_uncertainty_score":0.4436375,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.02408214294884004,"score_gpt":0.3092146191761493,"score_spread":0.2851324762273093,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}