{"id":"W4391315694","doi":"10.1021/acscatal.3c04931","title":"Functional Assessment of the Lewis Acid Strength of Structurally Complex Solid Acids","year":2024,"lang":"en","type":"article","venue":"ACS Catalysis","topic":"Zeolite Catalysis and Synthesis","field":"Chemistry","cited_by":22,"is_retracted":false,"has_abstract":true,"ca_institutions":"University of Toronto","funders":"Natural Sciences and Engineering Research Council of Canada; University of Toronto; Suncor Energy Incorporated","keywords":"Lewis acids and bases; Chemistry; Acid strength; Catalysis; Organic chemistry","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":["insufficient_payload"],"consensus_categories":[],"category_scores_codex":[0.000175465,0.0002078607,0.0004459965,0.0001048304,0.00008825579,0.00005198442,0.0004879785,0.00010559,0.003327336],"category_scores_gemma":[0.00007448571,0.0001405656,0.0006647013,0.0005353952,0.0001882491,0.0001394046,0.0002134233,0.0002084483,0.00001091924],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0000872613,"about_ca_system_score_gemma":0.0001564916,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00008305593,"about_ca_topic_score_gemma":0.0000302842,"domain_scores_codex":[0.9982314,0.00002954875,0.0005644259,0.0003546092,0.0006098998,0.000210125],"domain_scores_gemma":[0.9985481,0.0001695262,0.0002066103,0.0008712891,0.0001465319,0.00005796753],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.000008917304,0.00007696648,0.006810984,0.0003306498,0.001560047,0.000002860518,0.0002533669,0.0001503577,0.972374,0.001656086,0.001504499,0.01527125],"study_design_scores_gemma":[0.0001627126,0.00001080065,0.03277963,0.00008360379,0.000971764,0.000009606372,0.0004227801,0.002099321,0.9594057,0.0003107369,0.003533663,0.0002096455],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9900885,0.0005585268,0.0001456459,0.0004065803,0.0001336837,0.00004570036,0.0005297699,0.00004948054,0.008042154],"genre_scores_gemma":[0.9976178,0.00003416941,0.0003096846,0.00002515929,0.0001105222,0.0000129558,0.0005489032,0.00002397998,0.001316804],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.02596865,"threshold_uncertainty_score":0.9975837,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.02132421555035337,"score_gpt":0.2732465724658291,"score_spread":0.2519223569154758,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}