{"id":"W4400806604","doi":"10.1016/s1872-2067(24)60059-8","title":"Manipulating the interactions between N-intermediates and one-dimensional conjugated coordination polymers to boost electroreduction of nitrate to ammonia","year":2024,"lang":"en","type":"article","venue":"CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION)","topic":"Ammonia Synthesis and Nitrogen Reduction","field":"Chemical Engineering","cited_by":16,"is_retracted":false,"has_abstract":false,"ca_institutions":"University of Alberta","funders":"","keywords":"Conjugated system; Ammonia; Nitrate; Polymer; Chemistry; Combinatorial chemistry; Inorganic chemistry; Organic chemistry","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0004112599,0.0002449661,0.0004547151,0.0006384442,0.0001471561,0.00007232909,0.0001928142,0.00006605311,0.0000985294],"category_scores_gemma":[0.000438044,0.0001523542,0.0002580936,0.001123061,0.00004980626,0.0004716385,0.00008630995,0.0003585395,0.00002742194],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0001382052,"about_ca_system_score_gemma":0.00005728168,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0001447109,"about_ca_topic_score_gemma":0.00002902017,"domain_scores_codex":[0.99841,0.00006021076,0.0006959901,0.0002269798,0.0004088561,0.0001979774],"domain_scores_gemma":[0.9986916,0.0004020571,0.0002544316,0.0001700737,0.0002833062,0.0001985304],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.000228302,0.00006032465,0.01137633,0.00006690277,0.0006714233,0.000007098884,0.0007097753,0.003131447,0.9779551,0.00005837865,0.0002211955,0.005513742],"study_design_scores_gemma":[0.001534098,0.0007685616,0.1744185,0.001512104,0.002059276,0.0007842041,0.001312079,0.05502044,0.7593524,0.001156989,0.0009860502,0.001095288],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9943883,0.0004737564,0.001418228,0.003018445,0.0004758629,0.0001329873,0.0000219288,0.00003533734,0.00003519192],"genre_scores_gemma":[0.998378,0.00001292905,0.0007576337,0.00003560641,0.0005665555,0.000005079666,0.00003814855,0.0000336507,0.0001724184],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.2186027,"threshold_uncertainty_score":0.6212822,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.008960643914564668,"score_gpt":0.2588515125434064,"score_spread":0.2498908686288418,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}