{"id":"W4401459727","doi":"10.1021/acs.jpcc.4c04226","title":"Photo-Induced Force Microscopy-Based Spectroscopy and Chemical Mapping of Grafted Electrochemically Reduced Aryl Diazonium Salts","year":2024,"lang":"en","type":"article","venue":"The Journal of Physical Chemistry C","topic":"Force Microscopy Techniques and Applications","field":"Physics and Astronomy","cited_by":7,"is_retracted":false,"has_abstract":true,"ca_institutions":"Université du Québec à Montréal","funders":"Natural Sciences and Engineering Research Council of Canada; Canada Research Chairs; Canada Foundation for Innovation","keywords":"Monolayer; Microscopy; Diazonium Compounds; Infrared spectroscopy; Scanning probe microscopy; Scanning electrochemical microscopy; Aryl; Fourier transform infrared spectroscopy; Chemistry; Infrared microscopy; Materials science; Chemical force microscopy; Surface modification; Spectroscopy; Chemical imaging; Substrate (aquarium); Chemical engineering; Micrometer; Analytical Chemistry (journal); Electrochemistry; Nanotechnology; Conductive atomic force microscopy; Atomic force microscopy; Organic chemistry; Optics; Physical chemistry; Electrode; Non-contact atomic force microscopy","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001774712,0.0002335641,0.0003723489,0.00003223778,0.00006816854,0.00004854472,0.0003646067,0.00006242414,0.00005512448],"category_scores_gemma":[0.000009851911,0.0001708857,0.0002488372,0.0002965013,0.0001694229,0.00007282629,0.00006336399,0.0005941488,0.000002255207],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.00005320682,"about_ca_system_score_gemma":0.0001764633,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00001502394,"about_ca_topic_score_gemma":3.772773e-8,"domain_scores_codex":[0.9988467,0.00001572371,0.0004358302,0.0002003868,0.0002119018,0.0002894207],"domain_scores_gemma":[0.9990613,0.000171885,0.0002632711,0.0002669376,0.00011404,0.0001225195],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00007053684,0.0001390387,0.00002231704,0.0001093372,0.00007791608,9.293742e-7,0.000148973,0.000004926062,0.9984316,0.0002549075,0.0005432916,0.0001961962],"study_design_scores_gemma":[0.000282626,0.00008091108,0.00001374392,0.0002376118,0.00010778,0.00001187302,0.00006900947,0.001442848,0.9938436,0.003516243,0.0002299089,0.0001638785],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.994635,0.0001426301,0.003933203,0.0003583392,0.00002523288,0.0001445373,0.00002676272,0.00003425091,0.0007000563],"genre_scores_gemma":[0.9980742,0.000006413219,0.00128194,0.00002953154,0.0004800626,0.0000116022,0.00001626156,0.00003272852,0.00006730707],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.004588065,"threshold_uncertainty_score":0.6968515,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.006018975151363596,"score_gpt":0.2649520707031732,"score_spread":0.2589330955518096,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}