{"id":"W4401786549","doi":"10.1021/acsaem.4c01289","title":"Operando Three-Electrode Analysis of Nafion-Based Polymer Electrolyte Membrane Water Electrolyzers – Thermodynamic Relations","year":2024,"lang":"en","type":"article","venue":"ACS Applied Energy Materials","topic":"Hybrid Renewable Energy Systems","field":"Energy","cited_by":13,"is_retracted":false,"has_abstract":true,"ca_institutions":"Dalhousie University","funders":"Natural Sciences and Engineering Research Council of Canada; Research Nova Scotia; Canada Foundation for Innovation; Killam Trusts; CMC Microsystems","keywords":"Electrolyte; Nafion; Anode; Electrode; Cathode; Proton exchange membrane fuel cell; Polarization (electrochemistry); Materials science; Hydrogen production; Membrane; Electrolysis of water; Chemical engineering; Electrochemistry; Electrolysis; Hydrogen; Membrane electrode assembly; Chemistry; Organic chemistry","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0002058919,0.0002647528,0.0002796532,0.0003081835,0.0002306793,0.0003973358,0.0004225443,0.0003231002,0.0008802786],"category_scores_gemma":[0.0002765505,0.0001572169,0.0002624399,0.0002891377,0.000289352,0.0003935262,0.0002356069,0.0004829324,0.0001843441],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002384389,"about_ca_system_score_gemma":0.0001286896,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0007392569,"about_ca_topic_score_gemma":0.001238762,"domain_scores_codex":[0.9998566,0.00001357385,0.00001060431,0.00003006073,0.00006883463,0.00002030977],"domain_scores_gemma":[0.9999022,0.00003916819,0.00001378625,0.00001399554,0.0000256623,0.000005136774],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00003308534,0.00001941481,0.0007603235,0.00003715943,0.000008105207,0.00006375969,0.00005525655,0.000857854,0.9940322,0.0002958388,0.00003379602,0.003803242],"study_design_scores_gemma":[0.00000158786,0.00003805557,0.002263381,0.000001519313,0.000005240969,0.00004596283,0.00003785699,0.009735428,0.9873577,0.0001066864,0.0004024801,0.000004105751],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9782777,0.0002519768,0.01983532,0.00005167944,0.000009355085,0.00001906724,0.0002518024,0.0001767065,0.001126367],"genre_scores_gemma":[0.9945793,0.0001654324,0.00468422,0.000008556225,0.000002796336,0.00001551411,0.0001144787,0.00001953704,0.0004100577],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0008802786,"threshold_uncertainty_score":0.002944827,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.004890925709828074,"score_gpt":0.2024265838222248,"score_spread":0.1975356581123967,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}