{"id":"W4401997661","doi":"10.1021/acs.chemmater.4c00859","title":"Resorcinol–Azodianiline Covalent Organic Framework Supported FeOOH Quantum Dot-Catalyzed Electrochemical Ammonia Synthesis under Ambient Conditions","year":2024,"lang":"en","type":"article","venue":"Chemistry of Materials","topic":"Covalent Organic Framework Applications","field":"Materials Science","cited_by":1,"is_retracted":false,"has_abstract":true,"ca_institutions":"Carbon Engineering (Canada)","funders":"Air Force Office of Scientific Research; Core Research for Evolutional Science and Technology; Japan Society for the Promotion of Science; Indian Institute of Science Education and Research Pune; Ministry of Education, India; Council of Scientific and Industrial Research, India; Science and Engineering Research Board; Japan Student Services Organization; Department of Science and Technology, Ministry of Science and Technology, India","keywords":"Electrocatalyst; Heteroatom; Catalysis; Covalent bond; Aqueous solution; Covalent organic framework; Chemical engineering; Materials science; Electrochemistry; Imine; Inorganic chemistry; Chemistry; Nanotechnology; Organic chemistry; Electrode; Alkyl; Physical chemistry","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.000143463,0.0003444752,0.0002622683,0.0001264349,0.0001117307,0.0001748213,0.0003670064,0.0002538367,0.0006033274],"category_scores_gemma":[0.0001100366,0.0001199793,0.0001718655,0.0001112764,0.000127981,0.0002102997,0.000170849,0.000226391,0.0002243425],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0002935085,"about_ca_system_score_gemma":0.0001286895,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0008169175,"about_ca_topic_score_gemma":0.002455038,"domain_scores_codex":[0.9998139,0.00001695838,0.00001062407,0.00005996316,0.0000524545,0.00004625493],"domain_scores_gemma":[0.9999523,0.000007741809,0.00001179684,0.000008610797,0.0000105401,0.000009045586],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00001654739,0.0000145604,0.00006032671,0.00003433404,0.000005023289,0.00004602076,0.000008713701,0.0001181362,0.9976224,0.0001598599,0.00002856486,0.001885453],"study_design_scores_gemma":[0.000003933903,0.00003818854,0.0002811976,0.000001450788,0.000004245462,0.00004672488,0.00000466448,0.0008742445,0.9979133,0.00001524842,0.0008132975,0.00000338219],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9755308,0.001156678,0.01859789,0.00006987819,0.00005205996,0.00006986546,0.0002597235,0.0003691462,0.003893888],"genre_scores_gemma":[0.9898357,0.0003364518,0.008170003,0.00001265475,0.000006762898,0.00001938206,0.0001168523,0.00001637062,0.001485816],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0008169175,"threshold_uncertainty_score":0.002129555,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.01365078283431809,"score_gpt":0.2654004231795739,"score_spread":0.2517496403452558,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}