{"id":"W4403136672","doi":"10.1038/s41557-024-01650-6","title":"Hydrophobic assembly of molecular catalysts at the gas–liquid–solid interface drives highly selective CO2 electromethanation","year":2024,"lang":"en","type":"article","venue":"Nature Chemistry","topic":"CO2 Reduction Techniques and Catalysts","field":"Energy","cited_by":34,"is_retracted":false,"has_abstract":false,"ca_institutions":"Regroupement Québécois sur les Matériaux de Pointe; Université de Montréal","funders":"","keywords":"Chemistry; Catalysis; Electrochemistry; Dissolution; Terpyridine; Electrolyte; Cobalt; Chemical engineering; Electrode; Alkyl; Nanotechnology; Inorganic chemistry; Organic chemistry; Physical chemistry; Materials science","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.00008975959,0.0001752172,0.0001911732,0.0001375436,0.0002651196,0.0003802336,0.0002265454,0.0002106929,0.002064699],"category_scores_gemma":[0.0001894333,0.0002069626,0.0001064086,0.0001123492,0.0003252113,0.0003791908,0.0005048828,0.0004163627,0.0004864239],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0003414159,"about_ca_system_score_gemma":0.0001364359,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0003739576,"about_ca_topic_score_gemma":0.001337034,"domain_scores_codex":[0.9998925,0.00001111014,0.000004135558,0.00001819835,0.00003024271,0.00004378449],"domain_scores_gemma":[0.9998904,0.00003236764,0.00002378082,0.00001308668,0.00001155559,0.0000286982],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.0001068212,0.00004126919,0.0002205004,0.00003976647,0.000004914323,0.00009716336,0.00005573294,0.000587877,0.9946318,0.001205877,0.0002229413,0.002785428],"study_design_scores_gemma":[0.0000245329,0.0001321451,0.001018852,0.000003043739,0.000004285054,0.00003818962,0.0000601171,0.01113802,0.9853259,0.0001724566,0.002074305,0.00000812593],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9949899,0.0001469358,0.001914276,0.00009809418,0.00002353389,0.000007642231,0.00001624326,0.00006788878,0.002735472],"genre_scores_gemma":[0.9983469,0.00005645174,0.0004173586,0.00001633528,0.000007998073,0.000003822396,0.00001664533,0.00001453852,0.001119951],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.002064699,"threshold_uncertainty_score":0.006907105,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.003127500520441464,"score_gpt":0.2565166988903589,"score_spread":0.2533891983699175,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}