{"id":"W4403934791","doi":"10.1021/jacs.4c12385","title":"Coassembling Mesoporous Zeolitic Imidazolate Frameworks by Directed Reticular Chemistry","year":2024,"lang":"en","type":"article","venue":"Journal of the American Chemical Society","topic":"Metal-Organic Frameworks: Synthesis and Applications","field":"Chemistry","cited_by":10,"is_retracted":false,"has_abstract":true,"ca_institutions":"Canadian Light Source (Canada); University of British Columbia","funders":"H2020 Marie Skłodowska-Curie Actions; European Research Council; Killam Trusts; British Columbia Knowledge Development Fund; Natural Sciences and Engineering Research Council of Canada; Canada Research Chairs; Canada Foundation for Innovation; UK Research and Innovation","keywords":"Chemistry; Zeolitic imidazolate framework; Mesoporous material; Imidazolate; Reticular connective tissue; Nanotechnology; Metal-organic framework; Organic chemistry; Catalysis; Adsorption","routes":{"ca_aff":true,"ca_fund":true,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"metacan-v3-hybrid-931329e0061c","candidate_categories":[],"consensus_categories":[],"category_scores_codex":[0.0001134102,0.0004557871,0.0001713572,0.0002015346,0.0001298134,0.0002146613,0.0003359613,0.0002248456,0.0005919783],"category_scores_gemma":[0.0001618266,0.0001882106,0.0002160769,0.0000978215,0.0001661921,0.0002947786,0.0001853818,0.0002759079,0.0003178907],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.000282568,"about_ca_system_score_gemma":0.000136874,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.0004083484,"about_ca_topic_score_gemma":0.001231686,"domain_scores_codex":[0.9999064,0.000009019682,0.00000573087,0.00002895454,0.00002212595,0.00002771888],"domain_scores_gemma":[0.9999322,0.00001116741,0.00003325611,0.000009453537,0.000006402418,0.000007505629],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.00002096699,0.00001375584,0.00007854606,0.00004234442,0.000008016535,0.00003927979,0.00001682969,0.0003514402,0.9957146,0.0005057559,0.00007805879,0.003130305],"study_design_scores_gemma":[0.000008723138,0.00009642617,0.0004184835,0.000002167748,0.000006504966,0.00007488652,0.000004796836,0.00173373,0.9951546,0.00003811677,0.00245457,0.000006838594],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.9633877,0.002217016,0.02881418,0.00008441497,0.00005862241,0.0001180456,0.0003063097,0.0007924878,0.004221206],"genre_scores_gemma":[0.9796675,0.0007960706,0.01778645,0.00003484062,0.00001681474,0.00005034553,0.0001500943,0.00004225617,0.001455625],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0005919783,"threshold_uncertainty_score":0.002050221,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.006759550946589159,"score_gpt":0.2442204109366837,"score_spread":0.2374608599900945,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}