{"id":"W6989140506","doi":"","title":"Alteration of Electronic Band Structure &lt;i&gt;via &lt;/i&gt;a Metal-Semiconductor Interfacial Effect Enables High Faradaic Efficiency for Electrochemical Nitrogen Fixation","year":2021,"lang":"en","type":"article","venue":"Technical University of Denmark, DTU Orbit (Technical University of Denmark, DTU)","topic":"Ammonia Synthesis and Nitrogen Reduction","field":"Chemical Engineering","cited_by":0,"is_retracted":false,"has_abstract":false,"ca_institutions":"Discovery Centre","funders":"","keywords":"Faraday efficiency; Electrochemistry; Electrode; Nitrogen; Electronic structure","routes":{"ca_aff":true,"ca_fund":false,"ca_venue":false,"about_ca":false,"invisible_to_affiliation_only":false},"retraction":null,"screen":null,"direct_labels":[],"prediction":{"model_version":"codex-gemma-dda1882f352a","candidate_categories":["metaepi_narrow","insufficient_payload"],"consensus_categories":[],"category_scores_codex":[0.0005131329,0.0005661043,0.001344133,0.0003940915,0.0002887043,0.00001804817,0.001057624,0.0009991308,0.00107502],"category_scores_gemma":[0.0004472137,0.0006746913,0.0008759523,0.001000698,0.0006511557,0.0004159276,0.0003849305,0.0007713847,0.0000151599],"about_ca_system_candidate":false,"about_ca_system_consensus":false,"about_ca_system_score_codex":0.0007627282,"about_ca_system_score_gemma":0.0003528683,"about_ca_topic_candidate":false,"about_ca_topic_consensus":false,"about_ca_topic_score_codex":0.00008411863,"about_ca_topic_score_gemma":0.000281162,"domain_scores_codex":[0.9964659,0.0002528046,0.0007114874,0.0009971468,0.0007556101,0.0008170241],"domain_scores_gemma":[0.9969606,0.0007568357,0.0006931293,0.0006815552,0.0006486024,0.00025923],"domain_codex":null,"domain_gemma":null,"domain_candidate":null,"domain_consensus":null,"study_design_codex":"bench_or_experimental","study_design_gemma":"bench_or_experimental","study_design_scores_codex":[0.001570081,0.000411979,0.00006824385,0.0002919603,0.0003435169,0.0000205942,0.00006780362,0.0001667324,0.9915266,0.004056036,0.0004735809,0.001002874],"study_design_scores_gemma":[0.002450584,0.0007325956,0.0003735328,0.0002002285,0.0009416649,0.00008531208,0.0001045695,0.001923596,0.988767,0.001278194,0.002501219,0.0006415513],"study_design_candidate":"bench_or_experimental","study_design_consensus":"bench_or_experimental","genre_codex":"empirical","genre_gemma":"empirical","genre_scores_codex":[0.909017,0.001059132,0.0880194,0.0001592982,0.0000923108,0.0008154193,0.000181692,0.0001650292,0.0004907066],"genre_scores_gemma":[0.9923474,0.0002613017,0.006627277,0.000009924618,0.00007697733,0.000001342098,0.0001882145,0.00005264298,0.000434913],"genre_candidate":"empirical","genre_consensus":"empirical","teacher_disagreement_score":0.0833304,"threshold_uncertainty_score":0.9998381,"prediction_status":"machine_predicted_unvalidated"},"machine_scores":{"provisional":true,"baseline":true,"maturity_gate_passed":false,"score_opus":0.005246020408789309,"score_gpt":0.1865539524193342,"score_spread":0.1813079320105449,"validation_status":"score_only:v0-immature-baseline","note":"Baseline scores from an immature model (maturity gate not passed). Scores rank; they never assert a category."}}