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Hydrogen by Catalytic Steam Reforming of Liquid Byproducts from Biomass Thermoconversion Processes

2002· article· en· 451 citations· W1978988445 on OpenAlex· 10.1021/ie020107q

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Opus teacher head0.048
GPT teacher head0.251
Teacher spread
0.204 · how far apart the two teachers sit on this one work
Validation status
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Abstract

Biomass, a product of photosynthesis, is a renewable resource that can be used for sustainable production of hydrogen. We propose an approach that combines production of hydrogen with valuable coproducts and shows promising economics. The concept is based on a two-stage process: fast pyrolysis of biomass to generate bio-oil, followed by catalytic steam reforming of the bio-oil, or a fraction thereof, to produce hydrogen. The preferred option is separation of the bio-oil into a lignin-derived fraction, which could be used for producing phenolic resins or fuel-blending components, and a carbohydrate-derived material, which would be reformed to produce hydrogen. The coproduct strategy can also be applied to residual fractions derived from pulping operations or ethanol production and to effluents from other biomass conversion technologies such as transesterification of vegetable oils or food processing residues. In addition, all of the biomass-derived liquids can be coprocessed with natural gas to produce hydrogen from mixed fossil−biomass feedstocks, a strategy similar to cofiring biomass and coal for power generation. This work focuses on the second stage of the process: catalytic steam reforming of various biomass-derived liquids. We have used a commercial nickel-based naphtha reforming catalyst in a fluidized-bed reactor to produce hydrogen from the various biomass-derived liquids. Yields have approached or exceeded 80% of those theoretically possible for stoichiometric conversion.

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The record

Venue
Industrial & Engineering Chemistry Research
Topic
Thermochemical Biomass Conversion Processes
Field
Engineering
Canadian institutions
Funders
Université de SherbrookeU.S. Department of Energy
Keywords
Steam reformingBiomass (ecology)Hydrogen productionBiofuelBiomass to liquidNaphthaWaste managementChemistryLignocellulosic biomassPulp and paper industryHydrogenCatalysisChemical engineeringOrganic chemistry
Has abstract in OpenAlex
yes