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A simple effective potential for exchange

2006· article· en· 1,585 citations· W1996845210 on OpenAlex· 10.1063/1.2213970

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Abstract

The optimized effective potential (OEP) for exchange was introduced some time ago by Sharp and Horton and by Talman and Shadwick. The integral equation for the OEP is difficult to solve, however, and a variety of approximations have therefore been proposed. These are explicitly orbital dependent and require the same two-electron integrals as Hartree-Fock theory. We have found a remarkably simple approximate effective potential that closely resembles the Talman-Shadwick potential in atoms. It depends only on total densities and requires no two-electron integrals.

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The record

Venue
The Journal of Chemical Physics
Topic
Advanced Chemical Physics Studies
Field
Physics and Astronomy
Canadian institutions
Queen's University
Funders
Keywords
Simple (philosophy)Hartree–Fock methodElectronVariety (cybernetics)Computational chemistryPotential methodPhysicsQuantum mechanicsStatistical physicsChemistryMathematicsAlgorithm
Has abstract in OpenAlex
yes