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Record W2063177163 · doi:10.1021/es9907764

Solid-Solution Partitioning of Metals in Contaminated Soils:  Dependence on pH, Total Metal Burden, and Organic Matter

2000· article· en· W2063177163 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueEnvironmental Science & Technology · 2000
Typearticle
Languageen
FieldEnvironmental Science
TopicHeavy metals in environment
Canadian institutionsMcGill UniversityInstitut National de la Recherche Scientifique
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsEnvironmental chemistryMetalCadmiumSoil waterChemistryZincOrganic matterCopperSoil contaminationContaminationBioavailabilitySoil organic matterDissolved organic carbonSoil scienceEnvironmental scienceEcology

Abstract

fetched live from OpenAlex

Environmental risk assessment of metals depends to a great extent on modeling the fate and the mobility of metals based on soil−liquid partitioning coefficients. A large variability is observed among the reported values that could be used to predict metal mobility and bioavailability. To evaluate this, soil−liquid partitioning coefficients ( K d ) for many elements but especially for the metals cadmium, copper, lead, nickel, and zinc were compiled from over 70 studies of various origins collected from the literature. The relationships between the reported values are explored relative to variations in soil solution pH, soil organic matter (SOM), and concentrations of total soil metal. The results of multiple linear regressions show that K d values are best predicted using empirical linear regressions with pH (with R 2 values of 0.29−0.58) or with pH and either the log of SOM or the log of total metal and with resulting R 2 values of 0.42−0.76. A semi-mechanistic model based on the competitive adsorption of metal and H + [dependent on solution pH, total metal content, and log(SOM)] was a better tool to predict dissolved metal concentrations (with R 2 values of 0.61−0.88), with the exception of Pb (at 0.35).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.361
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.004
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0170.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.235
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it