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Record W2081909694 · doi:10.1021/ef9000242

Oil Characterization from Simulation of Experimental Distillation Data

2009· article· en· W2081909694 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueEnergy & Fuels · 2009
Typearticle
Languageen
FieldEngineering
TopicProcess Optimization and Integration
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsBoiling pointBubble pointDistillationFraction (chemistry)Vacuum distillationMole fractionMass fractionChemistryNaphthaBoilingBubbleThermodynamicsCharacterization (materials science)Molar massSpecific gravityChromatographyMaterials scienceMineralogyOrganic chemistryComputer scienceNanotechnologyCatalysisPhysical chemistry

Abstract

fetched live from OpenAlex

The characterization of crude oil involves dividing the oil into pseudocomponents and allocating mole fractions, molar mass, specific gravity, average boiling point, and critical properties to each component. The characterization is typically based on distillation data reported in terms of true boiling points. Standard assay types such as the ASTM D86 or ASTM D1160 vacuum distillation do not provide well established saturated bubble temperatures and require empirical interconversion curves to convert the assay data into true boiling point (TBP) data. Recently developed assays such as the ASTM D5236 and Bruno’s new distillation assay methodology do provide well-defined saturated bubble temperatures that correspond to actual thermodynamic state points but lack an established interconversion method to a TBP, that is, a method to determine the TBP of the fluid based on the measured temperatures of the assay. In this work, a methodology is presented to determine pseudocomponent mole fractions that match the boiling point data from these new assays. The fluid is divided into pseudocomponents of different average boiling point, and the molar mass and other physical properties of each component are determined using established correlations. A simulation of the distillation is optimized to match the assay data by adjusting the mole fraction of each pseudocomponent. The characterization can also be constrained to match other data such as the bulk density and molar mass of the fluid. The proposed methodology is tested on naphtha and Alaska crude oil and then verified through three heavy oil case studies. The methodology is entirely general and can be applied to a compositional analysis from a distillation of any material.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.559
Threshold uncertainty score0.347

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.248
Teacher spread0.230 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it