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Record W2330978563 · doi:10.1021/jp206011m

Application of the Multisolute Osmotic Virial Equation to Solutions Containing Electrolytes

2011· article· en· W2330978563 on OpenAlexafffund
Richelle C. Prickett, Janet A.W. Elliott, Locksley E. McGann

Bibliographic record

VenueThe Journal of Physical Chemistry B · 2011
Typearticle
Languageen
FieldChemistry
TopicElectrostatics and Colloid Interactions
Canadian institutionsUniversity of Alberta
FundersCanadian Institutes of Health Research
KeywordsElectrolyteVirial coefficientOsmotic coefficientThermodynamicsChemistryPitzer equationsAqueous solutionDebye–Hückel equationActivity coefficientVirial theoremPhysical chemistryPhysics

Abstract

fetched live from OpenAlex

The prediction of multisolute solution behavior of solutions containing electrolytes is important in many areas of research, including cryopreservation. In this study, the use of a novel form of the osmotic virial equation for multisolute solutions containing an electrolyte is investigated and compared to a rigorous electrolyte solution theory, the Pitzer-Debye-Huckel equation. For aqueous solutions containing a small molecule (either dimethyl sulfoxide or glycerol) and sodium chloride, the multisolute osmotic virial equation, which utilizes only two parameters to capture the electrolyte solution behavior, is shown to be as accurate as the Pitzer-Debye-Huckel equation, which utilizes six empirical parameters and multiple functions to capture the electrolyte solution behavior. In addition, an approach based on the multisolute osmotic virial equation to investigate the effect of electrolyte concentration on macromolecule solution behavior is presented and applied to aqueous solutions of hydroxyethyl starch and sodium chloride. The multisolute osmotic virial equation is shown to be an accurate, straightforward predictive solution theory for important multisolute solutions containing electrolytes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.003
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.003
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.250
Teacher spread0.228 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations45
Published2011
Admission routes2
Has abstractyes

Explore more

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