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Record W2589997655 · doi:10.1021/acsenergylett.6b00716

Outdoor Performance and Stability of Boron Subphthalocyanines Applied as Electron Acceptors in Fullerene-Free Organic Photovoltaics

2017· article· en· W2589997655 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Energy Letters · 2017
Typearticle
Languageen
FieldEngineering
TopicOrganic Electronics and Photovoltaics
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of British ColumbiaUniversity of Toronto
KeywordsOrganic solar cellMaterials scienceFullerenePhotovoltaicsElectron acceptorHeterojunctionBoronPhotovoltaic systemNanotechnologyChemical stabilityChemical engineeringOptoelectronicsChemistryComposite materialOrganic chemistryPolymerElectrical engineering

Abstract

fetched live from OpenAlex

The outdoor lifetime and performance of organic photovoltaics (OPVs) using boron subphthalocyanine (BsubPc) derivatives as electron-accepting materials is presented. The protocols followed are based on the most advanced level of outdoor testing established by the International Summit on OPV Stability (ISOS). The stability of each BsubPc is compared using three different sets of encapsulated planar heterojunction OPVs, with each set containing a different BsubPc as the electron-accepting layer. The performance and stability of each set is tested outdoors using an epoxy glue and a glass coverslip as protection from the ambient environment. Outdoor testing continued until the OPVs reached 80 or 50% of their original power conversion efficiency, as determined by frequent indoor characterization. OPVs utilizing chloro-BsubPc are shown to exhibit the highest stability and performance, while the stability of the other two BsubPc derivatives is reduced presumably as a result of their phenoxy or phenyl functionalization in the molecular axial positions. The established structure–property relationship and guidance for the design of future compounds for application in planar heterojunction OPVs are contrary to, and could not have been anticipated from, time zero laboratory testing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.190
Teacher spread0.184 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it