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Record W3168581589

Heteroatomic Jet Fuel Components: Lichen Substances as Fuel Component and Potential Additives

2016· article· en· W3168581589 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueNOT FOUND REPOSITORY (Indian Institute of Science Bangalore) · 2016
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicLichen and fungal ecology
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsJet fuelChemistryFourier transform ion cyclotron resonanceElectrospray ionizationMass spectrometryOrganic chemistryAnalytical Chemistry (journal)Chromatography
DOInot available

Abstract

fetched live from OpenAlex

This article presents chemical analysis of jet fuel (Jet A-1) heteroatomic fuel components with identification of an antioxidant lichen substance, gyrophoric acid in methanol extracted fuel samples. Thermal stressing of jet fuel produces soluble macromolecular oxidatively reactive species (SMORS) and heteroatomic deposits. SMORS are deposit precursors and elementary heteroatomic units containing unsaturated and aromatic hydrocarbons. Fuel additives such as antioxidants can inhibit SMORS and deposit formation within limited heating residence time and temperature range. Jet A-1 was thermally stressed in the autoxidation regime (150 to 300 0C) followed by spectroscopic analysis. Thermally stressed jet fuel static tests electrospray ionization mass spectra (ESI-MS) show higher molecular weight compounds in the mass range 300-1000 Da compared with unstressed fuel samples supporting deposition. Jet A-1 samples were analyzed by electrospray ion source mass spectrometry (ESI-MS), Fourier transform infrared (FTIR) and 13C nuclear magnetic resonance (NMR) spectroscopy. FTIR bands for oxygen containing species reveal the presence of alcohol, phenol and ether groups. 13C nuclear magnetic resonance (NMR) standard and distorsionless enhancement polarization transfer (DEPT 135) spectra recorded heteroatomic alkoxy species in both unstressed and thermally stressed fuel samples. Natural products polyphenols and lichen derived oxygenated compounds are excellent antioxidants. A new perspective of using lichen substances as fuel additives emerged in this study. Exploring further, natural products extraction methods optimization remains a key challenge and advantages of polyphenolic lichen acids as potential fuel and chemical additives are discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesScience and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.901
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.005
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.214
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it