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Record W4206953802 · doi:10.1515/tsd-2020-2305

Synthesis of multi-alkylpolyamines and their performance as flow improver in crude oil

2022· article· en· W4206953802 on OpenAlexaff
Zhichao Zhou, Sanbao Dong, Xiaolong Zhang, Jie Zhang, Hua Song, Gang Chen

Bibliographic record

VenueTenside Surfactants Detergents · 2022
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Calgary
FundersXi'an Shiyou UniversityNational Natural Science Foundation of China
KeywordsPour pointChemistryWaxAlkylCrude oilTriethylenetetramineDiethylenetriamineCrystallizationChromatographyOrganic chemistryNuclear chemistry

Abstract

fetched live from OpenAlex

Abstract In this work, three multi-alkyl polyamines, i.e., pentahexadecyl diethylenetriamine (PHDETA), hexahexadecyl triethylenetetramine (HHTETA) and heptahexadecyl tetraethylenepentylamine (HHTEPA), were synthesized and evaluated as pure flow improvers for crude oil. Under certain conditions, PHDETA, HHTETA and HHTEPA were able to improve the flow properties of L401 crude oil samples by reducing the viscosity of the crude oil by 97.5%, 94.3% and 97.1%, respectively. The three synthesized alkyl polyamines PHDETA, HHTETA and HHTEPA were able to reduce the viscosity of L1316 crude oil to a maximum of 94.3%, 93.7% and 94.9%, respectively. The pour point of L401 crude oil could be greatly reduced by 3.1 °C, 3.3 °C and 3.4 °C with PHDETA, HHTETA and HHTEPA, respectively. The pour point of L1316 crude oil with PHDETA, HHTETA and HHTEPA was strongly decreased by 2.8 °C, 2.9 °C and 3.2 °C, respectively. Photomicrographs showed the co-crystallization of L401 and L1316 crude oil in the presence of PHDETA, resulting in the formation of a non-close-packed network of wax crystals. The multi-alkyl polyamines have multiple alkyl side chains that extend in different directions into the oil phase and can co-crystallize with the wax molecules, allowing the wax crystals to disperse.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.225
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2022
Admission routes1
Has abstractyes

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