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Record W4212893393 · doi:10.1073/pnas.2113947119

Pharmaceutical pollution of the world’s rivers

2022· article· en· W4212893393 on OpenAlexafffund
John L. Wilkinson, Alistair B.A. Boxall, Dana W. Kolpin, Kmy Leung, Racliffe Weng Seng Lai, Cristóbal Galbán‐Malagón, Aiko D. Adell, Julie Mondon, Marc Métian, Rob Marchant, Alejandra Bouzas‐Monroy, Aida Cuní‐Sanchez, Anja Coors, Pedro Carriquiriborde, Macarena Rojo, Christopher Gordon, Magdalena Cara, Monique Moermond, Thais Luarte, Vahagn Petrosyan, Yekaterina Perikhanyan, Clare S. Mahon, Christopher J. McGurk, Thilo Hofmann, Tapos Kormoker, Volga Iñiguez, Jessica Guzman-Otazo, Jean Leite Tavares, Francisco Gildasio De Figueiredo, María Tereza Pepe Razzolini, Victorien Dougnon, Gildas Gbaguidi, Oumar Traoré, Jules M. Blais, Linda E. Kimpe, Michelle Wong, Donald Wong, Romaric Ntchantcho, Jaime Pizarro, Guang‐Guo Ying, Chang-Er Chen, Martha Isabel Páez-Melo, Jina Martínez-Lara, Jean‐Paul Otamonga, John Poté, Suspense A. Ifo, Penelope Wilson, Silvia Echeverría-Sáenz, Nikolina Udiković‐Kolić, Milena Milaković, Despo Fatta‐Kassinos, Lida Ioannou‐Ttofa, Vladimíra Belušová, Jan Vymazal, María Cárdenas-Bustamante, Bayable A. Kassa, Jeanne Garric, Arnaud Chaumot, Peter Gibba, Ilia Kunchulia, Sven Seidensticker, Gérasimos Lyberatos, Halldór Pálmar Halldórsson, Molly Melling, Shashidhar Thatikonda, Manisha Lamba, Anindrya Nastiti, Adee Supriatin, Nima Pourang, Ali Abedini, Omar Abdullah, Salem Gharbia, Francesco Pilla, Benny Chefetz, Tom Topaz, Koffi Marcellin Yao, Bakhyt Aubakirova, Raikhan Beisenova, Lydia Olaka, Jemimah K. Mulu, Peter Chatanga, Victor Ntuli, Nathaniel T. Blama, Sheck Sherif, Ahmad Zaharin Aris, Ley Juen Looi, Mahamoudane Niang, Seydou T. Traore, Rik Oldenkamp, Olatayo Michael Adetayo Ogunbanwo, Muhammad Ashfaq, Muhammad Iqbal, Ziad Abdeen, Aaron O’Dea, Jorge Manuel Morales‐Saldaña, María Custodio, Heidi De la Cruz, Ian A. Navarrete, Fábio Carvalho, Alhaji Brima Gogra, Bashiru M. Koroma, Vesna Cerkvenik‐Flajs, Mitja Gombač, Melusi Thwala, Kyungho Choi, Habyeong Kang, John Leju Celestino Ladu, Andreu Rico, Priyanie Amerasinghe, Anna Sobek, Gisela Horlitz, Armin Zenker, Alex C. King, Jheng‐Jie Jiang, Rebecca Kariuki, Madaka Tumbo, Ulaş Tezel, Turgut T. Onay, Julius B. Lejju, Yuliya Vystavna, Yuriy Vergeles, Horácio Heinzen, Andrés Pérez‐Parada, Douglas B. Sims, Maritza Figy, David A. Good, Charles Teta

Bibliographic record

VenueProceedings of the National Academy of Sciences · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicPharmaceutical and Antibiotic Environmental Impacts
Canadian institutionsUniversity of GuelphUniversity of Ottawa
FundersSchool of Public Health, Imperial College LondonInstitute of HydrobiologySmithsonian Tropical Research InstituteUniversidade de São PauloU.S. Geological SurveyNorthwestern UniversitySeoul National UniversityNazarbayev UniversityMbarara University of Science and TechnologyAgencia Nacional de Investigación y DesarrolloStockholms UniversitetInstitut chilien de l'AntarctiqueUniversiti Putra MalaysiaMedical Research CouncilUniversity of CyprusPatuakhali Science and Technology UniversityUniverza v LjubljaniIndian Institute of Technology DelhiAddis Ababa UniversityUniversidad del ValleKarolinska InstitutetČeská Zemědělská Univerzita v PrazeUniversity of GhanaNational and Kapodistrian University of AthensNational Technical University of AthensIranian Fisheries Science Research InstituteHebrew University of JerusalemKingston UniversityAkademie Věd České RepublikyUniversität WienUniversity of GujratMinistry of Education, IndiaChung Yuan Christian UniversityInternational Atomic Energy AgencyUniversité de GenèveSouth China Normal UniversityHáskóli ÍslandsDeakin UniversityUniversity of Dar es SalaamUniversity of OttawaImperial College LondonBritish CouncilUniversidad Nacional de La PlataUniversity College DublinUniversidad de Santiago de ChileUniversiteit van AmsterdamCity University of Hong KongSmithsonian Institution
KeywordsPollutionScale (ratio)Environmental scienceGeographyAquatic ecosystemDeveloping countryEnvironmental protectionEnvironmental healthEnvironmental resource managementEcologyBiologyCartographyMedicine

Abstract

fetched live from OpenAlex

Environmental exposure to active pharmaceutical ingredients (APIs) can have negative effects on the health of ecosystems and humans. While numerous studies have monitored APIs in rivers, these employ different analytical methods, measure different APIs, and have ignored many of the countries of the world. This makes it difficult to quantify the scale of the problem from a global perspective. Furthermore, comparison of the existing data, generated for different studies/regions/continents, is challenging due to the vast differences between the analytical methodologies employed. Here, we present a global-scale study of API pollution in 258 of the world's rivers, representing the environmental influence of 471.4 million people across 137 geographic regions. Samples were obtained from 1,052 locations in 104 countries (representing all continents and 36 countries not previously studied for API contamination) and analyzed for 61 APIs. Highest cumulative API concentrations were observed in sub-Saharan Africa, south Asia, and South America. The most contaminated sites were in low- to middle-income countries and were associated with areas with poor wastewater and waste management infrastructure and pharmaceutical manufacturing. The most frequently detected APIs were carbamazepine, metformin, and caffeine (a compound also arising from lifestyle use), which were detected at over half of the sites monitored. Concentrations of at least one API at 25.7% of the sampling sites were greater than concentrations considered safe for aquatic organisms, or which are of concern in terms of selection for antimicrobial resistance. Therefore, pharmaceutical pollution poses a global threat to environmental and human health, as well as to delivery of the United Nations Sustainable Development Goals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score0.023

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.003
Science and technology studies0.0010.000
Scholarly communication0.0010.001
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.055
GPT teacher head0.333
Teacher spread0.278 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1,509
Published2022
Admission routes2
Has abstractyes

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Same venueProceedings of the National Academy of SciencesSame topicPharmaceutical and Antibiotic Environmental ImpactsFrench-language works237,207