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Record W4221105210 · doi:10.1002/ese3.1107

The application of nonthermal plasma in methanol synthesis via CO<sub>2</sub> hydrogenation

2022· article· en· W4221105210 on OpenAlexafffund
Majid D. Farahani, Yimin Zeng, Ying Zheng

Bibliographic record

VenueEnergy Science & Engineering · 2022
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsNatural Resources CanadaWestern University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsCatalysisMethaneRenewable energyMethanolCombustionGasolineProcess engineeringNonthermal plasmaChemistryEnvironmental scienceNanotechnologyChemical engineeringMaterials sciencePlasmaOrganic chemistryEngineeringPhysics

Abstract

fetched live from OpenAlex

Abstract CH 3 OH is an energy carrier that can be generated from renewable resources and be used as a fuel in fuel cells and internal combustion engines and a platform chemical for the synthesis of value‐added chemicals or gasoline. Carbon dioxide (CO 2 ) hydrogenation is one of the widely researched methods to generate methanol. The traditional CO 2 hydrogenation reaction method (requires high H 2 pressure and temperatures) has attracted considerable attention. However, the new emerging field of catalysis referred to as nonthermal plasma (NTP) catalysis has also been developed extensively for methane reforming and CO 2 hydrogenation to methane and CO. The plasma‐assisted approach not only presents remarkable advantages, such as room temperature and atmospheric H 2 pressure but also has great potential to be powered by renewable electricity in a flexible way since it can be easily switched on/off. In this account, we review the recent articles published on methanol synthesis from CO 2 and H 2 using NTP. We reviewed and discussed the mechanism of this reaction under NTP, the modification of the reactor configurations, and the rationale behind the catalyst design. In the end, we discussed the advantages and disadvantages of each of these works and the future perspectives of this interesting privileged reaction. We believe this review is of interest to researchers active in sustainable heterogeneous catalysis.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.202
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2022
Admission routes2
Has abstractyes

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