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Record W4221126895 · doi:10.3389/fmats.2022.835855

Conductive, Anti-Corrosion, Self-Healing Smart Coating Technology Incorporating Graphene-Based Nanocomposite Matrix

2022· article· en· W4221126895 on OpenAlexaff
Jaime Benavides, Debika Banerjee, Dawit Gedamu, Luis Felipe Gerlein, Sylvain G. Cloutier

Bibliographic record

VenueFrontiers in Materials · 2022
Typearticle
Languageen
FieldMaterials Science
TopicSurface Modification and Superhydrophobicity
Canadian institutionsÉcole de Technologie Supérieure
Fundersnot available
KeywordsMaterials scienceChromate conversion coatingCorrosionGrapheneSalt spray testCoatingConversion coatingNanocompositeEnvironmentally friendlyElectrical resistance and conductanceComposite materialNanotechnologyRaman spectroscopySelf-healingElectrical conductorMetallurgyOptics

Abstract

fetched live from OpenAlex

Chromate conversion coatings have been in service for decades providing robust corrosion protection to a wide variety of aluminum alloys. However, it is also known that anti-corrosive coatings containing Cr6+ contributes to DNA damage, cause cancer and are not environmentally friendly. Consequently, regulatory restrictions over the use Cr6+ were established to mitigate the environmental damage and health problems. To answer to this hurdle and to meet the emergent need for environmentally friendly anti-corrosive coatings, we have successfully developed an innovative coating that combines anti-corrosive, low electrical resistance, and self-healing properties. First, we present two different coatings, that aim to display low electrical resistance properties: one containing only graphene and the other containing Zn nanoparticles and graphene. Confocal laser imaging and SEM microscopy was used to observe the morphology of the coatings. The electrical resistance was measured using the 4-wire connection Kelvin method. We compare the anticorrosive response for both coatings under neutral salt spray test (NSSt). Raman spectroscopy was performed before and after to understand the effect of NSSt corrosive species on the coatings. Then, we select the coating with lower electrical resistance, and we program on it a self-healing mechanism to boost its life service. Finally cyclic voltammetry is performed to confirm the excellent blocking properties of the tested coatings. All the coatings presented in this work are applied on aluminum AA 2024T351 and the optimal spray parameters for nanofillers dispersion are obtained. Our findings show great potential for preventing corrosion and compatibility with fully automated large-scale applications in different fields such as aerospace, automotive, construction, submarines and many more.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.242
Teacher spread0.230 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2022
Admission routes1
Has abstractyes

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