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Record W4254582392 · doi:10.1002/0471440264.pst141

Fractionation

2004· other· en· W4254582392 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueEncyclopedia of Polymer Science and Technology · 2004
Typeother
Languageen
FieldChemistry
TopicAnalytical Chemistry and Chromatography
Canadian institutionsUniversity of Waterloo
Fundersnot available
KeywordsFractionationPolymerComonomerChemistryChromatographyField flow fractionationElutionSize-exclusion chromatographyEquilibrium fractionationIsotope fractionationMaterials scienceAnalytical Chemistry (journal)PolymerizationOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Polymer fractionation techniques attempt to fractionate polymers according to specific characteristics of their microstructures as defined by their distributions of molecular weight, chemical composition, comonomer sequence length, tacticity, and long‐chain branching. Because of the heterogeneous nature of polymers, fractionation techniques are essential for understanding structure‐property relationships, polymerization mechanisms and kinetics, and polymer reaction engineering. In this entry, theoretical models to describe the microstructure of polymers are initially reviewed and used as a basis to understand the several polymer fractionation techniques described in the subsequent sections. Batch fractionation methods are covered next, including temperature variation and solvent/nonsolvent fractionation procedures. The recent technique of crystallization analysis fractionation (Crystaf), together with temperature rising elution fractionation (TREF), are reviewed as methods for fractionation by crystallizability. The well‐established technique for molecular weight fractionation by size‐exclusion chromatography (SEC) is covered next, followed by a section on the versatile field flow fractionation (FFF). Large‐scale fractionation of polymers is covered in the section for continuous polymer fractionation (CPF). Mass spectrometry, particularly matrix‐assisted laser desorption ionization coupled with time‐of‐flight analyzers (MALDI‐TOF) is the subject of the next section. Finally, a section in interaction chromatography and some other less general polymer fractionation techniques is followed by the concluding section on cross‐fractionation techniques.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.294
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.002
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.221
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it